This research investigated the ablation process of commercial stainless steels with ultrashort pulsed laser. Square hollows were ablated on stainless steel sheets using a picosecond laser with pulse duration of 0.25, 1 and 10 ps, respectively, and fluence ranging from 0.125 J/cm 2 to 5 J/cm 2 . For each setting the surface quality and ablation efficiency were determined by optical microscopy and scanning electron microscopy (SEM). Processing windows producing high quality surfaces at high ablation efficiency were found at a fluence around 0.75 J/cm 2 for the two shorter pulse lengths tested. Individual cones and periodic cone-like protrusions were found in the low fluence regime (< 0.625 J/cm 2 ) and high fluence regime (> 0.875 J/cm 2 ), respectively, both of which make the ablated surface rough. Emphasizing on the individual cones, it is found that the cones are caused by inclusions in the base materials, attributed to a higher fluence threshold required for ceramic-like inclusions. This novel theory explaining the creation mechanism is verified by multiple analysis methods like SEM and energy dispersive X-ray spectroscopy and stop-motion SEM imaging. current hypotheses are self-organization as suggested by Reif et al. [14]
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