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We report the fabrication and properties of soft glass photonic crystal fibers (PCF's) for supercontinuum generation. The fibers have zero or anomalous group velocity dispersion at wavelengths around 1550 nm, and approximately an order of magnitude higher nonlinearity than attainable in comparable silica fibers. We demonstrate the generation of an ultrabroad supercontinuum spanning at least 350 nm to 2200 nm using a 1550 nm ultrafast pump source.

We report the fabrication of a Tellurite photonic crystal fiber, and demonstrate its waveguiding properties. The measured minimum loss is 2.3 dB/m at a wavelength of 1055 nm. The fiber supports several modes, but in practice just the fundamental mode can be used. We have observed strong stimulated Raman scattering in a fiber with an effective area Aeff=21.2microm2, using sub-ns, ~ 1 microJ pump pulses at 1064.

The conversion of light fields in photonic crystal fibers (PCFs) capitalizes on the dramatic enhancement of several optical nonlinearities. We present here spectrally smooth, highly broadband supercontinuum radiation in a short piece of high-nonlinearity soft-glass PCF. This supercontinuum spans several optical octaves, with a spectral range extending from 350 nm to beyond 3000 nm. The selection of an appropriate propagation-length determines the spectral quality of the supercontinuum generated. Experimentally, we clearly identify two regimes of nonlinear pulse transformation: when the fiber length is much shorter than the dispersion length, soliton propagation is not important and a symmetric supercontinuum spectrum arises from almost pure self-phase modulation. For longer fiber lengths the supercontinuum is formed by the breakup of multiple Raman-shifting solitons. In both regions very broad supercontinuum radiation is produced.

Third order nonlinear optical characterization of bismuth zinc borate glasses are reported here using different laser pulse durations. Bismuth zinc borate glasses with compositions xBi2O3-30ZnO-(70-x) B2O3 (where x = 30, 35, 40, and 45 mol. %) have been prepared by melt quenching method. These glasses were characterized by Raman, UV-Vis absorption, and Z scan measurements. Raman and UV-Vis spectroscopic results indicate that non-bridging oxygens increase with increase of bismuth content in the glass. Nonlinear absorption and refraction behavior in the nanosecond (ns), picosecond (ps), and femtosecond (fs) time domains were studied in detail. Strong reverse saturable absorption due to dominant two-photon absorption (TPA) was observed with both ps and fs excitations. In the case of ns pulse excitations, TPA and free-carrier absorption processes contribute for the nonlinear absorption. Two-photon absorption coefficient (β) and the absorption cross section due to free carriers (σe) are estimated by theoretical fit of the open aperture Z-scan measurements and found to be dependent on the amount of bismuth oxide in the glass composition. In both ns and fs regimes the sign and magnitude of the third order nonlinearity are evaluated, and the optical limiting characteristics are also reported.

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