The feasibility of a novel technique for efficient and selective population transfer from a thermally populated level 1 via an intermediate state 2 to level 3 is experimentally demonstrated. It is shown for sodium dimers that the process of on- or near-resonance stimulated Raman scattering with only partially overlapping laser beams is, in particular, useful for the selective population of high vibrational levels of particles in a molecular beam. This is achieved when the interaction with the Stokes laser, coupling levels 2 and 3, begins earlier than the interaction with the pump laser. The phenomenon, which is closely related to the formation of ‘‘trapped states,’’ is quantitatively explained using the basis of eigenstates of molecules strongly coupled to the radiation fields. The similarity and difference to related techniques such as rapid adiabatic passage phenomena in two-level systems, off-resonant stimulated Raman scattering, or stimulated emission pumping is briefly discussed.

Kuklinski, J. R.; Gaubatz, U.; Hioe, Foek T.; and Bergmann, K (1989). "Adiabatic population transfer in a three-level system driven by delayed laser pulses. " Physical Review A 40.11,[6741][6742][6743][6744] Please note that the Publication Information provides general citation information and may not be appropriate for your discipline. To receive help in creating a citation based on your discipline, please visit http://libguides.sjfc.edu/citations.Adiabatic population transfer in a three-level system driven by delayed laser pulses AbstractWe give a simple analytic solution that describes a novel method for population transfer in a three-level system driven by delayed pulses and which accounts for recent experimental results. This solution describes a procedure that is counter intuitive, and yet it is shown to be, in fact, one of the simplest solutions for multilevel systems arising from the adiabatic theorem. Its possible application to many-level systems is suggested. We give a simple analytic solution that describes a novel method for population transfer in a three-level system driven by delayed pulses and which accounts for recent experimental results. This solution describes a procedure that is counterintuitive, and yet it is shown to be, in fact, one of the simplest solutions for multilevel systems arising from the adiabatic theorem. Its possible application to many-level systems is suggested. Disciplines Physics

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A broadband technique for robust adiabatic rotation and conversion of light polarization is proposed. It uses the analogy between the equation describing the polarization state of light propagating through an optically anisotropic medium and the Schrödinger equation describing coherent laser excitation of a three-state atom. The proposed technique is analogous to the stimulated Raman adiabatic passage (STIRAP) technique in quantum optics; it is applicable to a wide range of frequencies and it is robust to variations in the propagation length and the rotary power.