We report superior terahertz parametric generation from potassium titanyl phosphate (KTP) over congruent-grown lithium niobate (CLN) and lithium tantalate (CLT) in terms of parametric gain and laser damage resistance. Under the same pump and crystal configurations, the signal emerged first from KTP, 5% Mg-doped CLN, CLN, and then finally from CLT. The signal growth rate in KTP was comparable to that in 5%-Mg-doped CLN, but the signal power from KTP reached a much higher value after all the other crystals were damaged by the pump laser. We further demonstrate seeded terahertz parametric amplification in an edge-cut KTP at 5.74 THz. The THz parametric amplifier (TPA) employs a 17-mm long KTP gain crystal, pumped by a passively Q-switched pump laser at 1064 nm and seeded by a continuous-wave diode laser tuned to the signal wavelength at 1086.2 nm. With 5.8-mJ energy in a 520-ps pump pulse and 100-mW seed signal power, we measured 5-W peak-power THz output from the KTP TPA with 22% pump depletion. In comparison, we measured no detectable THz output power from a similar edge-cut CLN TPA under the same pump power, detection scheme, and crystal configuration, when tuning the seed laser wavelength to 1072.2 nm and attempting to generate a radiation at 2.1 THz.
Optical parametric mixing is a popular scheme to generate an idler wave at THz frequencies, although the THz wave is often absorbing in the nonlinear optical material. It is widely suggested that the useful material length for co-directional parametric mixing with strong THz-wave absorption is comparable to the THz-wave absorption length in the material. Here we show that, even in the limit of the absorption loss exceeding parametric gain, the THz idler wave can grows monotonically from optical parametric amplification over a much longer distance in a nonlinear optical material until pump depletion. The coherent production of the non-absorbing signal wave can assist the growth of the highly absorbing idler wave. We also show that, for the case of an equal input pump and signal in difference frequency generation, the quick saturation of the THz idler wave predicted from a much simplified and yet popular plane-wave model fails when fast diffraction of the THz wave from the co-propagating optical mixing waves is considered.
Lithium niobate is the most popular material for terahertz wave generation via stimulated polariton scattering (SPS), previously known to have a gain peak near 2 THz. Here we report the discovery of another phase-matched gain peak near 4 THz in lithium niobate, which greatly extends the useful gain spectrum of lithium niobate. Despite the relatively high 4 THz absorption in lithium niobate, the 4 THz SPS becomes dominant over the 2 THz one in an intensely pumped short lithium niobate crystal due to less diffraction-induced absorption and mode-area mismatch. We also demonstrate a signal-seeded OTPO that generates 1.4 nJ at 4.2 THz from lithium niobate with 17.5 mJ pump energy.
scite is a Brooklyn-based organization that helps researchers better discover and understand research articles through Smart Citations–citations that display the context of the citation and describe whether the article provides supporting or contrasting evidence. scite is used by students and researchers from around the world and is funded in part by the National Science Foundation and the National Institute on Drug Abuse of the National Institutes of Health.