[1] A band of enhanced aerosol optical depth (AOD) over the mid-to-high latitude Southern Oceans exists in some passive satellite-based aerosol data sets, including Moderate Resolution Imaging Spectroradiometer (MODIS) products. Past studies suggest several potential causes contributing to this phenomenon, including signal uncertainty, retrieval bias, and cloud contamination. In this paper, quality-assured Aqua MODIS aerosol products in this zonal band are investigated to assess cloud contamination as a cause. Spatially and temporally collocated cloud and aerosol products produced by the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) project relative to Aqua MODIS AOD in this region are considered. Maritime Aerosol Network (MAN) and Aerosol Robotic Network (AERONET) AOD data are also collocated with Aqua MODIS retrievals for surface context. The results of this study indicate that the high Aqua MODIS AOD are not seen in the CALIOP aerosol products, cannot be screened using active profiling of collocated observations for cloud presence, and are not detected by ground-based observations such as MAN and AERONET. Enhanced AOD values are attributable primarily to stratocumulus and low broken cumulus cloud contamination, as identified with CALIOP products. But these clouds explain only about 30-40% of the total anomaly. Cirrus cloud contamination is also a factor. However, in contrast to the rest of the globe, they contribute less overall, relative to low-level liquid water clouds, which are considered likely the result of misidentification of relatively warm cloud tops compared with surrounding open seas.

Abstract. Data products from the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) on board Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) were recently updated following the implementation of new (version 4) calibration algorithms for all of the Level 1 attenuated backscatter measurements. In this work we present the motivation for and the implementation of the version 4 nighttime 532 nm parallel channel calibration. The nighttime 532 nm calibration is the most fundamental calibration of CALIOP data, since all of CALIOP's other radiometric calibration procedures – i.e., the 532 nm daytime calibration and the 1064 nm calibrations during both nighttime and daytime – depend either directly or indirectly on the 532 nm nighttime calibration. The accuracy of the 532 nm nighttime calibration has been significantly improved by raising the molecular normalization altitude from 30–34 km to the upper possible signal acquisition range of 36–39 km to substantially reduce stratospheric aerosol contamination. Due to the greatly reduced molecular number density and consequently reduced signal-to-noise ratio (SNR) at these higher altitudes, the signal is now averaged over a larger number of samples using data from multiple adjacent granules. Additionally, an enhanced strategy for filtering the radiation-induced noise from high-energy particles was adopted. Further, the meteorological model used in the earlier versions has been replaced by the improved Modern-Era Retrospective analysis for Research and Applications, Version 2 (MERRA-2), model. An aerosol scattering ratio of 1.01±0.01 is now explicitly used for the calibration altitude. These modifications lead to globally revised calibration coefficients which are, on average, 2–3 % lower than in previous data releases. Further, the new calibration procedure is shown to eliminate biases at high altitudes that were present in earlier versions and consequently leads to an improved representation of stratospheric aerosols. Validation results using airborne lidar measurements are also presented. Biases relative to collocated measurements acquired by the Langley Research Center (LaRC) airborne High Spectral Resolution Lidar (HSRL) are reduced from 3.6 %±2.2 % in the version 3 data set to 1.6 %±2.4 % in the version 4 release.

Abstract. Due to instrument sensitivities and algorithm detection limits, level 2 (L2) Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) 532 nm aerosol extinction profile retrievals are often populated with retrieval fill values (RFVs), which indicate the absence of detectable levels of aerosol within the profile. In this study, using 4 years (2007–2008 and 2010–2011) of CALIOP version 3 L2 aerosol data, the occurrence frequency of daytime CALIOP profiles containing all RFVs (all-RFV profiles) is studied. In the CALIOP data products, the aerosol optical thickness (AOT) of any all-RFV profile is reported as being zero, which may introduce a bias in CALIOP-based AOT climatologies. For this study, we derive revised estimates of AOT for all-RFV profiles using collocated Moderate Resolution Imaging Spectroradiometer (MODIS) Dark Target (DT) and, where available, AErosol RObotic NEtwork (AERONET) data. Globally, all-RFV profiles comprise roughly 71 % of all daytime CALIOP L2 aerosol profiles (i.e., including completely attenuated profiles), accounting for nearly half (45 %) of all daytime cloud-free L2 aerosol profiles. The mean collocated MODIS DT (AERONET) 550 nm AOT is found to be near 0.06 (0.08) for CALIOP all-RFV profiles. We further estimate a global mean aerosol extinction profile, a so-called “noise floor”, for CALIOP all-RFV profiles. The global mean CALIOP AOT is then recomputed by replacing RFV values with the derived noise-floor values for both all-RFV and non-all-RFV profiles. This process yields an improvement in the agreement of CALIOP and MODIS over-ocean AOT.

Abstract. The Cloud Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) mission released version 4.00 of their lidar level 1 data set in April of 2014, and subsequently updated this to version 4.10 in November of 2016. The primary difference in the newly released version 4 (V4) data is a suite of updated calibration coefficients calculated using substantially revised calibration algorithms. This paper describes the revisions to the V4 daytime calibration procedure for the 532 nm parallel channel. As in earlier releases, the V4 daytime calibration coefficients are derived by scaling the raw daytime signals to the calibrated nighttime signals acquired within a calibration transfer region, and thus the new V4 daytime calibration benefits from improvements made to the V4 532 nm nighttime calibration. The V4 calibration transfer region has been moved upward from the upper troposphere to the more stable lower stratosphere. The identification of clear-air columns by an iterative thresholding scheme, crucial to selecting the observation regions used for calibration, now uses uncalibrated 1064 nm data rather than recursively using the calibrated 532 nm data, as was done in version 3 (V3). A detailed account of the rationale and methodology for this new calibration approach is provided, along with results demonstrating the improvement of this calibration over the previous version. Extensive validation data acquired by NASA's airborne high spectral resolution lidar (HSRL) shows that during the daytime the average difference between collocated CALIPSO and HSRL measurements of 532 nm attenuated backscatter coefficients is reduced from 3.3 %±3.1 % in V3 to 1.0 %±3.5 % in V4.