The radiation transport effect on pellet implosion and the Rayleigh-Taylor (R-T) instability are studied in a light-ion beam (LIB) inertial confinement fusion (ICF) by numerical simulation and analytic work. First, we present the nonuniformity-smoothing effect of the radiation transport on implosion symmetry in an LIB ICF fuel pellet. The 2-D implosion simulation shows that the initial nonuniformity can be smoothed out well in an LIB ICF pellet; for example, the initial nonuniformity of 6% is smoothed to 0.07% during the implosion phase. In addition, linear analyses for the R-T instability under nonuniform acceleration in space and under radiation are also performed: The nonuniform acceleration field in space does not change the growth rate (γ) of the R-T instability. However, this nonuniformity may suppress the growth itself of the R-T instability. Radiation may reduc the growth rate (γ).
We use a 6.8-fs laser as the light source for broad-band femtosecond pump-probe real-time vibrational spectroscopy to investigate both electronic relaxation and vibrational dynamics of the Q(y)-band of Chl-a at 293 K. More than 25 vibrational modes coupled to the Q(y) transition are observed. Eleven of them have been clarified predominantly due to the excited state, and six of them are concluded to be nearly exclusively resulting from the ground-state wave-packet motion. Moreover, thanks to the broad-band detection over 5000 cm⁻¹, the modulated signals due to the excited state vibrational coherence are observed on both sides of the 0-0 transition with equal separation. The corresponding nonlinear process has been studied using a three-level model, from which the probe wavelength dependence of the phase of the periodic modulation can be calculated. The probe wavelength dependence of the vibrational amplitude is interpreted in terms of the interaction between the "pump" or "laser," Stokes, and anti-Stokes field intermediated by the molecular vibrations. In addition, an excited state absorption peak at ~709 nm has been observed. To the best of our knowledge, this is the first study of broad-band real-time vibrational spectroscopy in Chl-a.
We propose and demonstrate experimentally a novel way of generating sub-10fs deep-UV pulses. The technique is based on chirped-pulse four-wave mixing induced by a broadband near-IR (NIR) pulse and a near-UV pulse. The broadband IR pulse is prepared by preliminarily broadening the spectral width of an NIR pulse by self-phase modulation. The positively chirped broadband IR pulse is suitable for generating a negatively chirped deep-UV pulse, which can be compressed by normal group-velocity dispersion in a transparent medium. Self-compression of the generated deep-UV pulse in air has been demonstrated to produce sub-10fs deep-UV pulses with excellent temporal and spectral profiles for ultrafast spectroscopy in the deep UV.
Measurements and calculations of the contribution of the non-dipole terms in the angular distribution of photoelectrons from the K-shell of randomly oriented N2 molecules are reported. The angular distributions have been measured in the plane containing the photon polarization and the photon momentum vectors of linearly polarized radiation. Calculations have been performed in the relaxed core Hartree–Fock approximation with a fractional charge, and many-electron correlations were taken into account in the random phase approximation. Both theory and experiment show that the non-dipole effects are rather small in the photon energy region from the ionization threshold of the K-shell up to about 70 eV above it. From the theory, it follows that the non-dipole terms for the individual 1σg and 1σu shells are considerably large; therefore measurements resolving the contributions of the 1σg and 1σu shells are desirable.
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