A B S T R A C TThe isotopic composition of precipitation has been measured in samples simultaneously collected during individual precipitation events at two neighbouring high-altitude stations (Houxia at 2100 m a.s.l. and Gaoshan at 3545 m a.s.l.) in the Tianshan Mts., northwest China. The observed changes of δ 18 O (δ 2 H) and deuterium excess with surface air temperature, altitude and season have been evaluated to derive information on the effects of subcloud evaporation and moisture recycling on the formation of precipitation and its isotopic composition under arid climatic conditions. Consulting the long-term monthly averages of 'd' excess and temperature of the nearest GNIP station Wulumuqi, a striking similarity was found with the results of the two high-altitude stations concerning the relation between 'd' excess and temperature. The 'd' excess-temperature plot of the Wulumuqi data shows an hysteresis effect which appears to signify seasonal changes in the interplay between subcloud evaporation and moisture recycling. Finally, for the first time a negative altitude gradient of the d excess has been found for all stations including two more GNIP stations in northwest China but far away from the study area. This 'inverse altitude effect' may manifest a decrease of the recycled fraction in air moisture with altitude.
Soil and vadose zone profiles are used as an archive of changes in groundwater recharge and water quality following changes in land use in an area of the Loess Plateau of China. A typical rain-fed loess-terrace agriculture region in Hequan, Guyuan, is taken as an example, and multiple tracers (chloride mass balance, stable isotopes, tritium and water chemistry) are used to examine groundwater recharge mechanisms and to evaluate soil water chloride as an archive for recharge rate and water quality. Results show that groundwater recharge beneath natural uncultivated grassland, used as a baseline, is about 94-100 mm year À1 and that the time it takes for annual precipitation to reach water table through the thick unsaturated zone is from decades to hundreds of years (tritium free). This recharge rate is 2-3 orders of magnitude more than in the other semiarid areas with similar annual rainfall but with deep-rooted vegetation and relatively high temperature. Most of the water that eventually becomes recharge originally infiltrated in the summer months. The conversion from native grassland to winter wheat has reduced groundwater recharge by 42-50% (50-55 mm year À1 for recharge), and the conversion from winter wheat to alfalfa resulted in a significant chloride accumulation in the upper soil zone, which terminated deep drainage. The paper also evaluates the time lag between potential recharge and actual recharge to aquifer and between increase in solute concentration in soil moisture and that in the aquifer following land-use change due to the deep unsaturated zone.
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