The unique structural and physical properties of two-dimensional (2D) atomic layer semiconductors render them promising candidates for electronic or optoelectronic devices. However, the lack of efficient and stable approaches to synthesize large-area thin films with excellent uniformity hinders their realistic applications. In this work, we reported a method involving atomic layer deposition and a chemical vapor deposition chamber to produce few-layer 2H-MoSe2 thin films with wafer-level uniformity. The reduction of MoO3 was found indispensable for the successful synthesis of MoSe2 films due to the low vaporization temperature. Moreover, a metal-semiconductor-metal photodetector (PD) was fabricated and investigated systematically. We extracted an ultrahigh photoresponsivity approaching 101 A/W with concomitantly high external quantum efficiency up to 19,668% due to the produced gain arising from the holes trapped at the metal/MoSe2 interface, the band tail state contribution, and the photogating effect. A fast response time of 22 ms was observed and attributed to effective nonequilibrium carrier recombination. Additionally, the ultrahigh photoresponsivity and low dark current that originated from Schottky barrier resulted in a record-high specific detectivity of up to 2×1013 Jones for 2D MoSe2/MoS2 PDs. Our findings revealed a pathway for the development of high-performance PDs based on 2D MoSe2 that are inexpensive, large area, and suitable for mass production and contribute to a deep understanding of the photoconductivity mechanisms in atomically thin MoSe2. We anticipate that these results are generalizable to other layer semiconductors as well.
Subauroral proton arcs are a type of terrestrial auroral phenomena, which are often detached equatorially from the auroral oval. This work presents evolution of a subauroral proton arc using observations of the Special Sensor Ultraviolet Spectrographic Imager and Special Sensor J (SSJ) on board Defense Meteorological Satellite Program (DMSP) spacecraft. The arc was observed in the afternoon sector and was located within 60°–70° geomagnetic latitude during the recovery phase of a moderate magnetic storm with the minimum SYM‐H index of −55 nT. Particle measurements from DMSP F17/SSJ indicate that the arc was detached from the normal oval and produced by energetic ring current ions with energies above 10 keV. These energetic ions were likely scattered into the magnetic loss cone by electromagnetic ion cyclotron waves in the frequency range between 0.1 and 0.5 Hz, as confirmed by Pc1 waves derived from the observations of a ground station. Continuous auroral observations directly show that the subauroral proton arc was detached from the oval during evolution. Following a northward interplanetary magnetic field turning, the auroral oval moved toward higher latitudes. We propose that the equatorward edge of the auroral oval is less influenced by the convection electric field, and thus moves more slowly than the poleward edge. This mechanism is proposed for producing a separation between the equatorward and poleward parts of the auroral oval, with the former evolving into the subauroral proton arc.
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