Since the invention of optical tweezers, optical manipulation has advanced significantly in scientific areas such as atomic physics, optics and biological science. Especially in the past decade, numerous optical beams and nanoscale devices have been proposed to mechanically act on nanoparticles in increasingly precise, stable and flexible ways. Both the linear and angular momenta of light can be exploited to produce optical tractor beams, tweezers and optical torque from the microscale to the nanoscale. Research on optical forces helps to reveal the nature of light–matter interactions and to resolve the fundamental aspects, which require an appropriate description of momenta and the forces on objects in matter. In this review, starting from basic theories and computational approaches, we highlight the latest optical trapping configurations and their applications in bioscience, as well as recent advances down to the nanoscale. Finally, we discuss the future prospects of nanomanipulation, which has considerable potential applications in a variety of scientific fields and everyday life.
A multifocus optical vortex metalens, with enhanced signal-to-noise ratio, is presented, which focuses three longitudinal vortices with distinct topological charges at different focal planes. The design largely extends the flexibility of tuning the number of vortices and their focal positions for circularly polarized light in a compact device, which provides the convenience for the nanomanipulation of optical vortices.
Separating substances by their chirality faces great challenges as well as opportunities in chemistry and biology. In this study, we propose an all-optical solution for passive sorting of chiral objects using chirality-dependent lateral optical forces induced by judiciously interfered fields. First, we investigate the optical forces when the chiral objects are situated in the interference field formed by two plane waves with arbitrary polarization states. When the plane waves are either linearly or circularly polarized, nonzero lateral forces are found at the particle's trapping positions, making such sideways motions observable. Although the lateral forces have different magnitudes on particles with different chirality, their directions are the same for opposite handedness particles, rendering it difficult to separate the chiral particles. We further solve the sorting problem by investigating more complicated polarization states. Finally, we achieve the chiral-selective separation by illuminating only one beam toward the chiral substance situated at an interface between two media, taking advantage of the native interference between the incident and reflective beams at the interface. Our study provides a robust and insightful approach to sort chiral substances and biomolecules with plausible optical setups.
Lateral optical forces induced by linearly polarized laser beams have been predicted to deflect dipolar particles with opposite chiralities toward opposite transversal directions. These "chirality-dependent" forces can offer new possibilities for passive all-optical enantioselective sorting of chiral particles, which is essential to the nanoscience and drug industries. However, previous chiral sorting experiments focused on large particles with diameters in the geometrical-optics regime. Here, we demonstrate, for the first time, the robust sorting of Mie (size~wavelength) chiral particles with different handedness at an air-water interface using optical lateral forces induced by a single linearly polarized laser beam. The nontrivial physical interactions underlying these chirality-dependent forces distinctly differ from those predicted for dipolar or geometrical-optics particles. The lateral forces emerge from a complex interplay between the light polarization, lateral momentum enhancement, and out-of-plane light refraction at the particle-water interface. The sign of the lateral force could be reversed by changing the particle size, incident angle, and polarization of the obliquely incident light.
The determination of optical force as a consequence of momentum transfer is inevitably subject to the use of the proper momentum density and stress tensor. It is imperative and valuable to consider the intrinsic scheme of photon momentum transfer, particularly when a particle is embedded in a complex dielectric environment. Typically, we consider a particle submerged in an inhomogeneous background composed of different dielectric materials, excluding coherent illumination or hydrodynamic effects. A ray-tracing method is adopted to capture the direct process of momentum transfer from the complex background medium, and this approach is validated using the modified Einstein-Laub method, which uses only the interior fields of the particle in the calculation. In this way, debates regarding the calculation of the force with different stress tensors using exterior fields can be avoided. Our suggested interpretation supports only the Minkowski approach for the optical momentum transfer to the embedded scatterer while rejecting Peierls's and Abraham's approaches, though the momentum of a stably moving photon in a continuous background medium should be considered to be of the Abraham type. Our interpretation also provides a novel method of realizing a tractor beam for the exertion of negative force that offers an alternative to the use of negative-index materials, optical gain, or highly non-paraxial or multiple-light interference. Keywords: dielectric interface; Minkowski photon momentum transfer; modified Einstein-Laub method; optical pulling force; optical tractor beams INTRODUCTIONFollowing the pioneering work of Marston 1 in acoustics, optical 'tractor beams' have attracted considerable interest by virtue of their unusual mechanism for micromanipulation. [2][3][4][5][6][7][8][9][10][11][12][13] Generally speaking, a tractor beam is a customized light beam that exerts a negative scattering force (NSF) on a scatterer and pulls it opposite to the propagation direction of the light, in contrast to conventional pushing forces. 14 Optical pulling forces provide a novel approach to gradientless optical manipulation techniques distinct from optical tweezers, 15-17 optical conveyors 13,18,19 and nanooptomechanical systems. 20,21 Recently, various types of tractor beams have been experimentally demonstrated using a Gaussian beam with an optical mirror (involving the interference of incident and reflected light beams in certain limited regions) 8 and using dodecane droplets sitting on a dielectric interface. 22 However, in the presence of a high-powered laser, hydrodynamic effects (uneven heat dissipation, particle absorption, temperature gradients, liquid convection, surface energy wells, etc.) may also contribute. Moreover, the stability criteria for tractor beams, which are very important for practical application, have not yet been investigated.Although the mechanical effect has been demonstrated 22 to be an overall consequence of all possible contributing factors, the mechanism of the optical momentum transfer from a mixe...
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