Spintronic structures are extensively investigated for their spin–orbit torque properties, required for magnetic commutation functionalities. Current progress in these materials is dependent on the interface engineering for the optimization of spin transmission. Here, we advance the analysis of ultrafast spin-charge conversion phenomena at ferromagnetic-transition metal interfaces due to their inverse spin-Hall effect properties. In particular, the intrinsic inverse spin-Hall effect of Pt-based systems and extrinsic inverse spin-Hall effect of Au:W and Au:Ta in NiFe/Au:(W,Ta) bilayers are investigated. The spin-charge conversion is probed by complementary techniques—ultrafast THz time-domain spectroscopy in the dynamic regime for THz pulse emission and ferromagnetic resonance spin-pumping measurements in the GHz regime in the steady state—to determine the role played by the material properties, resistivities, spin transmission at metallic interfaces, and spin-flip rates. These measurements show the correspondence between the THz time-domain spectroscopy and ferromagnetic spin-pumping for the different set of samples in term of the spin mixing conductance. The latter quantity is a critical parameter, determining the strength of the THz emission from spintronic interfaces. This is further supported by ab initio calculations, simulations, and analysis of the spin-diffusion and spin-relaxation of carriers within the multilayers in the time domain, permitting one to determine the main trends and the role of spin transmission at interfaces. This work illustrates that time-domain spectroscopy for spin-based THz emission is a powerful technique to probe spin-dynamics at active spintronic interfaces and to extract key material properties for spin-charge conversion.
We report on theoretical investigations of scattering asymmetry vs. incidence of carriers through exchange barriers and magnetic tunnel junctions made of semiconductors involving spin-orbit interaction. By an analytical 2 × 2 spin model, we show that, when Dresselhaus interaction is included in the conduction band of antiparallel magnetized electrodes, the electrons can undergo a large difference of transmission depending on the sign of their incident in-plane wavevector. In particular, the transmission is fully quenched at some points of the Brillouin zone for specific in-plane wavevectors and not for the opposite. Moreover, it is universally scaled by a unique function independent of the spin-orbit strength. This particular feature is reproduced by a 14 × 14 band k · p model showing, in addition, corresponding effects in the valence band and highlighting the robustness of the effect, which even persists for a single magnetic electrode. Upon tunneling, electrons undergo an asymmetrical deflection which results in the occurrence of a transverse current, giving rise to a so-called Tunnel Hall Effect. arXiv:1509.00657v1 [cond-mat.mes-hall] 2 Sep 2015
Terahertz (THz) spin‐to‐charge conversion has become an increasingly important process for THz pulse generation and as a tool to probe ultrafast spin interactions at magnetic interfaces. However, its relation to traditional, steady state, ferromagnetic resonance techniques is poorly understood. Here, nanometric trilayers of Co/X/Pt (X = Ti, Au or an Au:W alloy) are investigated as a function of the “X” layer thickness, where THz emission generated by the inverse spin Hall effect is compared to the Gilbert damping of the ferromagnetic resonance. Through the insertion of the “X” layer it is shown that the ultrafast spin current injected in the non‐magnetic layer defines a direct‐spin‐conductance, whereas the Gilbert damping leads to an effective spin‐mixing‐conductance of the trilayer. Importantly, it is shown that these two parameters are connected to each other and that spin‐memory‐losses can be modeled via an effective Hamiltonian with Rashba fields. This work highlights that magneto‐circuit concepts can be successfully extended to ultrafast spintronic devices, as well as enhancing the understanding of spin‐to‐charge conversion processes through the complementarity between ultrafast THz spectroscopy and steady state techniques.
Topological insulator spin-polarized surface states are attractive for spintronic applications, in particular for spin-charge current interconversion, where extremely high conversion efficiencies are predicted. However, the contribution of topologically trivial bulk states is often disregarded although it may play a crucial role in the experimental results and extracted conversion efficiencies. The presence of bulk states at the Fermi level can be avoided by increasing the gap using the confinement effect appearing as the film thickness is reduced. We address this topic by growing Bi 1−x Sb x thin films (2.5-15 nm) by molecular beam epitaxy on InSb, BaF 2 , and Si substrates. The surface electronic band structure is studied by angle-resolved photoemission spectroscopy. Two Bi 1−x Sb x surface states are observed in the gap for several Sb concentrations and thicknesses, across the topological insulator phase, scanning x between 7% and 30%. Tight-binding calculations of the surface states are in good agreement with the experiments, revealing their polarized nature. Surface states are still present at the point for the thinnest films (2.5 nm), suggesting highly confined polarized states at the surface.
Teleost fish express highly diverse naive TCRβ (TRB) repertoires and mount strong public and private clonal responses upon infection with pathogens. Fish T cells express typical markers such as CD8, CD4-1 and CD4-2, CD3, CD28 and CTLA4. Fish CD8+ T cells have been shown to be responsible for antigen-specific cell-mediated cytotoxicity in in vitro systems using histo-compatible effector and target cells. We compare here the complexity of TRB repertoires between FACS sorted CD8+ and CD8− T cells from spleen and pronephros of rainbow trout. In contrast to human, while the TRB repertoire is highly diverse and polyclonal in CD8+ T cells of naïve fish, it appeared very different in CD8− lymphocytes with irregular CDR3 length distributions suggesting a dominance of activated clones already in naïve fish or the presence of non conventional T cells. After infection with a systemic virus, CD8+ T cells mount a typical response with significant skewing of CDR3 length profiles. The infection also induces significant modifications of the TRB repertoire expressed by the CD8− fraction, but for a different set of V/J combinations. In this fraction, the antiviral response results in an increase of the peak diversity of spectratypes. This unusual observation reflects the presence of a number of T cell expansions that rise the relative importance of minor peaks of the highly skewed distributions observed in unchallenged animals. These results suggest that the diversity of TRB expressed by CD8+ and CD8− αβ T cells may be subjected to different regulatory patterns in fish and in mammals.
The main purpose of this study is to complete the research process of dispersing nanoclay I.30E (montmorillonite) into epoxy Epikote 240 by mechanical method combined with energy-saving ultrasonic method. We investigate appropriate dispersion conditions such as stirring speed, mechanical stirring temperature, ultrasonic stirring time, and ultrasonic stirring capacity, which affect the mechanical properties and fire resistance of nanocomposite materials. The nanoclay contents studied were 1, 2, 3, and 4% by weight, and the methods used in this study are FE-SEM; XRD; and flame-retardant evaluation methods: LOI, UL 94HB. The mechanical properties were studied: tensile strength, flexural strength, compression strength, and impact resistance Izod. The dispersion method was recommended to stir mechanically at a speed of 3000 rpm at 80°C for 8 hours and then conduct ultrasonic vibrations for 6 hours at 65°C. The results showed that epoxy Epikote 240/nanoclay I.30E nanocomposite material had mechanical properties and improved fire retardancy with a small amount of nanoclay I.30E added (2% by weight): tensile strength of 63.5 MPa (increased by 13.59%), flexural strength of 116.80 MPa (increased by 34.63%), compressive strength of 179.67 MPa (increased by 15.11%), impact resistance Izod of 12.81 KJ/m2 (increased by 80.16%), oxygen limit of 23.7%, and combustion rate of 24.5 mm/min; according to UL 94HB, the combustion rate reached 22.59 mm/min.
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