Pyrogenic carbon, also called black carbon (BC), is an important component in the global carbon cycle. BC produced by biomass burning or fossil fuel combustion is transported to oceans by the atmosphere or rivers. However, environmental dynamics (i.e., major sources and sinks) of BC in marine environments have not been well-documented. In this study, dissolved BC (DBC) collected from surface waters of the Chukchi Sea, the Bering Sea, and the subarctic and subtropical North Pacific were analyzed using the benzene polycarboxylic acid (BPCA) method. The DBC concentration and the ratio of B5CA and B6CA to all BPCAs (an index of the DBC condensation degree) ranged from 4.8 to 15.5 µg-C L −1 and from 0.20 to 0.43, respectively, in surface waters of the Chukchi/Bering Seas and the North Pacific Ocean. The concentration and condensation degree of DBC in the Chukchi/Bering Seas were higher and more variable than those in the subarctic and subtropical North Pacific, which implies that the major factors controlling DBC distribution were different in these marine provinces. In the Chukchi/Bering Seas, the DBC concentration was negatively correlated to salinity but positively correlated to chromophoric dissolved organic matter (CDOM) quantity and total dissolved lignin phenol concentration estimated by CDOM parameters. These correlations indicated that the possible major source of DBC in the Chukchi/Bering Seas was Arctic rivers. However, in the North Pacific, where riverine inputs are negligible for most sampling sites, DBC was possibly derived from the atmosphere. Although spectral slopes of CDOM at 275-295 nm (an index of the photodegradation degree of CDOM) differed widely between the subarctic and subtropical North Pacific, the concentration and condensation degrees of DBC were similar between the subarctic and subtropical North Pacific, which suggests that photodegradation was not the only major factor controlling DBC distribution. Therefore, DBC distributions of the North Pacific Ocean were considered to be mainly controlled by atmospheric deposition of BC and subsequent losses by photodegradation and adsorption onto sinking particles. This study implies that the main influence on DBC distribution in the open ocean and the coastal ocean are atmospheric deposition and fluvial inputs, respectively.
19We investigated branched and isoprenoid glycerol dialkyl glycerol tetraethers (GDGTs) in 20 surface soils and a paleosol sequence to understand the effects of environmental and
Abstract. We generated a 280 000 yr record of water pH and temperature in Lake Biwa, central Japan, by analysing the methylation index (MBT ) and cyclisation ratio (CBT) of branched tetraethers in sediments from piston and borehole cores. Our aim was to understand the responses of precipitation and air temperature in central Japan to the East Asian monsoon variability on orbital timescales. Because the water pH in Lake Biwa is determined by phosphorus and alkali cation inputs, the record of water pH should indicate the changes in precipitation and temperature in central Japan. Comparison with a pollen assemblage in a Lake Biwa core suggests that lake water pH was determined by summer temperature in the low-eccentricity period before 55 ka, while it was determined by summer precipitation in the higheccentricity period after 55 ka. From 130 to 55 ka, the variation in lake pH (summer precipitation) lagged behind that in summer temperature by several thousand years. This perspective is consistent with the conclusions of previous studies (Igarashi and Oba, 2006;Yamamoto, 2009), in that the temperature variation preceded the precipitation variation in central Japan.
Sandy shelf sediments are important elements of clastic sedimentary systems because of their wide distribution in the geological record and their significance as hydrocarbon reservoirs. Although many studies have investigated shelf sediments influenced by waves or tidal currents, little is known about shelf sediments influenced by oceanic currents, particularly their lithofacies characteristics and stratigraphic evolution. This study investigated the stratigraphic evolution of shelf sediments off the Kujukuri strandplain facing the Pacific Ocean, which is influenced by the strong Kuroshio Current. Sediment cores were obtained from six locations on the Kujukuri shelf (34 to 124 m water depth) using a vibrocorer. The dominant lithofacies is mud‐free sand with low‐angle cross‐lamination associated with alternating beds of finer and coarser sand with cross‐lamination. These display depositional processes influenced by storm waves and the Kuroshio Current, respectively. This finding is consistent with the previously presented modern and historical observations of the Kuroshio Current and estimates of the storm‐wave base. Radiocarbon dates show that the sediment succession formed during the last transgressive and highstand stages after 13·1 ka. The depositional processes during the stages represent a transition from storm waves with abundant sediment supply to both storm waves and the Kuroshio Current with sediment starvation mainly due to its trapping in the strandplain. Comparison to other Holocene–Modern shelf systems suggests that the sandy shelf successions are strongly influenced by oceanic currents under conditions of limited riverine input and open coastal geometry. The resultant sand‐dominated succession is characterized by reversal of the proximal to distal grain‐size trend compared to the fining for most other recognized wave/storm‐dominated shelf successions. This is because of seaward increase in the influence of the Kuroshio Current. Thus, shelf deposits are naturally complex, and these may be further complicated by the additional influence of oceanic currents above the usual wave‐dominated and tide‐dominated end members.
Abstract. We generated a 282 000-year record of water pH and temperature in Lake Biwa, central Japan, by analysing the methylation index (MBT') and cyclisation ratio (CBT) of branched tetraethers in sediments from piston and borehole cores to understand the responses of precipitation and air temperature in central Japan to the East Asian monsoon variability on the orbital timescale. Because water pH in Lake Biwa is determined by phosphorus input driven by precipitation, the record of water pH should indicate changes in summer precipitation in central Japan. The estimated pH showed significant periodicity at 19 and 23 ka (precession) and at 41 ka (obliquity). The variation in the estimated pH agrees with variation in the pollen temperature index. This indicates synchronous variation in summer air temperature and precipitation in central Japan, which contradicts the conclusions of previous studies. The variation in estimated pH was also synchronous with the variation of oxygen isotopes in stalagmites in China, suggesting that East Asian summer monsoon precipitation was governed by Northern Hemisphere summer insolation on orbital timescales. However, the estimated winter temperatures were higher during interglacials and lower during glacials, showing an eccentricity cycle. This suggests that the temperature variation reflected winter monsoon variability.
scite is a Brooklyn-based organization that helps researchers better discover and understand research articles through Smart Citations–citations that display the context of the citation and describe whether the article provides supporting or contrasting evidence. scite is used by students and researchers from around the world and is funded in part by the National Science Foundation and the National Institute on Drug Abuse of the National Institutes of Health.