Helium films show various quantum phases that undergo quantum phase transitions by changing coverage n. We found anomalous elastic phenomena in bosonic 4 He and fermionic 3 He films adsorbed on a glass substrate. The films stiffen under AC strain at low temperature with an excess dissipation. The onset temperature of the stiffening decreases to 0 K as n approaches a critical coverage nc. The elastic anomaly is explained by thermal activation of helium atoms from the localized to extended states with a distributed energy gap. We determine for the first time the energy band structure of helium films from elasticity. The ground states of 4 He and 3 He at n < nc are identically gapped and compressible, which are possibly a sort of Mott insulator or Mott glass.
Magnetization dynamics induced by parametric excitation in a magnetic dot has been investigated by using ac spin pumping and inverse spin-Hall effects. An Ising-like pair of states with different precession phases was found to be stabilized in a controllable way under the excitation. The result shows that the dot can be used as a parametron-bit carrier. Upon increasing the excitation power, stochastic transition between the states was observed, and the occurrence probability of each state can be tuned by means of additional microwaves, opening an application to probabilistic bit operation.
Molecular hydrogen is a fascinating candidate for quantum fluid showing bosonic and fermionic superfluidity. We have studied diffusion dynamics of thin films of H2, HD and D2 adsorbed on a glass substrate by measurements of elasticity. The elasticity shows multiple anomalies well below bulk triple point. They are attributed to three different diffusion mechanisms of admolecules and their "freezing" into localized state: classical thermal diffusion of vacancies, quantum tunneling of vacancies, and diffusion of molecules in the uppermost surface. The surface diffusion is active down to 1 K, below which the molecules become localized. This suggests that the surface layer of hydrogen films is on the verge of quantum phase transition to superfluid state.
Thermoelectric effects have been applied to power generators and temperature sensors that convert waste heat into electricity. The effects, however, have been limited to electrons to occur, and inevitably disappear at low temperatures due to electronic entropy quenching. Here, we report thermoelectric generation caused by nuclear spins in a solid: nuclear-spin Seebeck effect. The sample is a magnetically ordered material MnCO3 having a large nuclear spin (I = 5/2) of 55Mn nuclei and strong hyperfine coupling, with a Pt contact. In the system, we observe low-temperature thermoelectric signals down to 100 mK due to nuclear-spin excitation. Our theoretical calculation in which interfacial Korringa process is taken into consideration quantitatively reproduces the results. The nuclear thermoelectric effect demonstrated here offers a way for exploring thermoelectric science and technologies at ultralow temperatures.
Adsorbed molecular films provide two-dimensional systems that show various emergent phenomena that are not observed in bulk counterparts. We have measured the elasticity of thin neon films adsorbed on porous glass down to 1 K by the torsional oscillator technique. The shear modulus of a neon film anomalously increases at low temperatures with excess dissipation. This behavior indicates a crossover from a soft (fluidlike) state at high temperatures to a stiff (solidlike) state at low temperatures. The temperature dependence of the anomaly is qualitatively similar to that of the elastic anomaly of helium films found in our recent study. The dissipation peak temperature, however, becomes constant at about 5 K, contrary to the case of helium, in which it decreases to 0 K at a critical coverage of a quantum phase transition between a gapped localized phase and a mobile (superfluid) phase. It is concluded that neon films behave as a classical system that does not show a quantum phase transition or superfluidity, although the films may be strongly supercooled to temperatures much lower than the bulk triple point, 24.6 K. Our results suggest that the elastic anomaly is a universal phenomenon of atomic or molecular films adsorbed on disordered substrates.
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