2021
DOI: 10.1038/s41467-021-24623-6
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Observation of nuclear-spin Seebeck effect

Abstract: Thermoelectric effects have been applied to power generators and temperature sensors that convert waste heat into electricity. The effects, however, have been limited to electrons to occur, and inevitably disappear at low temperatures due to electronic entropy quenching. Here, we report thermoelectric generation caused by nuclear spins in a solid: nuclear-spin Seebeck effect. The sample is a magnetically ordered material MnCO3 having a large nuclear spin (I = 5/2) of 55Mn nuclei and strong hyperfine coupling, … Show more

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Cited by 24 publications
(17 citation statements)
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“…In spin pumping via hyperfine interaction, g ↑↓ represents the rate of spin-flipped reflection of conduction electron near the magnetic interface. Although the conduction spin has quadrupole anisotropy, due to orthogonality of the terms inside the integral in (13), the nuclear ( 14) spin pumping is isotropic, similar to those of conventional exchange spin pumping, and its magnitude that depends on the hyperfine interaction strength, as observed in Ref. [8].…”
Section: Nuclear Spin Pumpingmentioning
confidence: 72%
See 1 more Smart Citation
“…In spin pumping via hyperfine interaction, g ↑↓ represents the rate of spin-flipped reflection of conduction electron near the magnetic interface. Although the conduction spin has quadrupole anisotropy, due to orthogonality of the terms inside the integral in (13), the nuclear ( 14) spin pumping is isotropic, similar to those of conventional exchange spin pumping, and its magnitude that depends on the hyperfine interaction strength, as observed in Ref. [8].…”
Section: Nuclear Spin Pumpingmentioning
confidence: 72%
“…Because of that, a better understanding of the mechanism spin transfer is required. Furthermore, a more efficient spin energy transfer may be achieved because nuclear spin has a lower excitation energy [13].…”
Section: Introductionmentioning
confidence: 99%
“…Fitting mathematical models to the experimental data has also been proposed as a method to identify the magnetic thermopower [255]. Clearly, measuring the transport properties as a function of the magnetic field is the best method to determine the magnetic thermopower [236,256,257].…”
Section: Magnetic Semiconductorsmentioning
confidence: 99%
“…in Figure 2 in the previous review article (2). Recent updates include ferromagnetic EuO (15), two-dimensional (2D) ferromagnetic Cr2Si2Te6, Cr2Ge2Te6 (16,17), ferrimagnetic garnet ferrites R3Fe5O12 (R = Eu, Tb, Dy, Tm) (18,19,20), Y3−xRxFe5O12 with R being 14 rare-earth elements from La to Lu (except for Pm) (21), Lu2Bi1Fe4Ga1O12 (22), spinel ferrites ZnFe2O4 (23), γ-Fe2O3 (24), LiFe5O8 (25), Ni0.65Zn0.35Al0.8Fe1.2O4 (26), Mg 0.5−δ Mn0.5Fe2O4 (27), Y-type hexagonal ferrites Ba2Co2Fe12O22, Ba2Zn2Fe12O22 (28), orthorhombic ferrimagnetic ε-Fe2O3 (29), molecular-based ferrimagnetic Cr II [Cr III (CN)6] (30), various antiferromagnetic (AF) insulators such as NiO (31,32,33,34), FeF2 (35), α-Fe2O3 (36,37), MnCO3 (38), α-Cu2V2O7 (39), SrFeO3 (40), SrMnO3 (41), DyFeO3 (42), and other intriguing materials including a chiral helimagnet Cu2OSeO3 with a skyrmion lattice phase (43,44) and quantum magnets Sr2CuO3 (45,46), CuGeO3 (47), Pb2V3O9 (48), LiCuVO4 (49). In particular, the ferrimagnetic insulator YIG has been essential (1,2), as it exhibits the lowest magnetic damping, high Curie temperature (TC ∼ 560 K), and high resistivity and also is a playground to reveal the role of magnon polarization in SSEs (see Section 6).…”
Section: Introductionmentioning
confidence: 99%