Proximity‐induced tuning of spin–orbit coupling (SOC) is of paramount importance in emerging magnetic materials and in spintronics. Probing the above SOC via light–matter interaction assisted methods provides a novel route to investigate interesting material phenomena. Here, the proximity studies in a heterostructure of monolayer molybdenum disulfide (MS) and iron (Fe) to enhance and tune the interfacial SOC are reported. The augmented SOC of the MSFe heterostructure arises due to interfacial charge transfer, and is probed using magneto‐optic Kerr effect and a novel optical technique utilizing the spin Hall effect of light. Measuring the changes in the state of polarization of light reflected from the sample via weak measurement provides direct access to the real and imaginary parts of the complex weak value and, hence, the underlying SOC and induced magnetic effects from a single experiment. The results obtained are confirmed using other experimental and simulation tools.

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A scheme to study the effect of residual phase gradients in an optical interference between two out-of-phase Gaussian beams is proposed. In a Sagnac interferometer configured to provide a null output, a variable linear phase swept across the null point unfolds an optical field rotation due to an apparently negligible residual phase gradient present orthogonal to the linear phase sweep. As the optical beam that rotates around its propagation axis carries orbital angular momentum, the experimental results presented in this Letter could provide an insight into the momentum change associated with the energy redistribution in the fundamental phenomenon of optical interference.

We propose a distinct concept on the generation of optical vortex through coupling between the amplitude and phase differences of the superposing beams. For the proof-of-concept demonstration, we propose a simple free-space optics recipe for the controlled synthesis of an optical beam with a vortex dipole by superposing two transversely scaled Gaussian beams. The experimental demonstration using a Sagnac interferometer introduces the desired amount of radial shear and linear phase difference between the two out-of-phase Gaussian beams to create a vortex pair of opposite topological charge in the superposed beam. Flexibility to tune their location and separation using the choice of direction of the linear phase difference and the amount of amplitude difference between the superposing beams has potential applications in optical tweezers and traps utilizing the local variation in angular momentum across the beam cross section.

Accumulation of geometric phase due to non-coplanar propagation of higher-order modes in an optical fiber is experimentally demonstrated. Vertically-polarized LP11 fiber mode, excited in a horizontally-held, torsion-free, step-index, two-mode optical fiber, rotates due to asymmetry in the propagating k-vectors, arising due to off-centered beam location at the fiber input. Perceiving the process as due to rotation of the fiber about the off-axis launch position, the orbital Berry phase accumulation upon scanning the launch position in a closed-loop around the fiber axis manifests as rotational Doppler effect, a consequence of orbit–orbit interaction. The anticipated phase accumulation as a function of the input launch position, observed through interferometry is connected to the mode rotation angle, quantified using the autocorrelation method.

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Simultaneous extraction of the magnetic and spin‐orbit coupling (SOC) information of an interface using the weak measurement assisted spin‐Hall effect of light (SHEL) is demonstrated as a novel probe to characterize materials' magnetic properties, see article number 2000042 by Karthik V. Raman, Tharangattu N. Narayanan, Nirmal K. Viswanathan, and co‐workers. A heterostructure of Fe and MoS2 monolayers is shown for enhanced SOC due to the proximity effect, which is proven via SHEL method and then confirmed using magneto‐optic Kerr effect (MOKE) studies.