We report our study of the evolution of superconductivity and the phase diagram of the ternary Fe(Se 1-x Te x ) 0.82 (0 ≤ x ≤ 1.0) system. We discovered a new superconducting phase with T c , max = 14 K in the 0.3 < x < 1.0 range. This superconducting phase is suppressed when the sample composition approaches the end member FeTe 0.82 , which exhibits an incommensurate antiferromagnetic order. We discuss the relationship between the superconductivity and magnetism of this material system in terms of recent results from neutron scattering measurements. Our results and analyses suggest that superconductivity in this new class of Fe-based compounds is associated with magnetic fluctuations, and therefore may be unconventional in nature.
The iron chalcogenide Fe(1+y)(Te(1-x)Se(x)) is structurally the simplest of the Fe-based superconductors. Although the Fermi surface is similar to iron pnictides, the parent compound Fe(1+y)Te exhibits antiferromagnetic order with an in-plane magnetic wave vector (pi,0) (ref. 6). This contrasts the pnictide parent compounds where the magnetic order has an in-plane magnetic wave vector (pi,pi) that connects hole and electron parts of the Fermi surface. Despite these differences, both the pnictide and chalcogenide Fe superconductors exhibit a superconducting spin resonance around (pi,pi) (refs 9, 10, 11). A central question in this burgeoning field is therefore how (pi,pi) superconductivity can emerge from a (pi,0) magnetic instability. Here, we report that the magnetic soft mode evolving from the (pi,0)-type magnetic long-range order is associated with weak charge carrier localization. Bulk superconductivity occurs as magnetic correlations at (pi,0) are suppressed and the mode at (pi, pi) becomes dominant for x>0.29. Our results suggest a common magnetic origin for superconductivity in iron chalcogenide and pnictide superconductors.
We have investigated the effect of Fe nonstoichiometry on properties of the Fe 1+y (Te, Se) superconductor system by means of resistivity, Hall coefficient, magnetic susceptibility, and specific heat measurements. We find that the excess Fe at interstitial sites of the (Te, Se) layers not only suppresses superconductivity, but also results in a weakly localized electronic state. We argue that these effects originate from the magnetic coupling between the excess Fe and the adjacent Fe square planar sheets, which favors a short-range magnetic order.
We have studied the coupling of electronic and magnetic properties in Fe1+y(Te1-xSex) via systematic specific heat, magnetoresistivity, and Hall coefficient measurements on two groups of samples with y = 0.02 and 0.1. In the y = 0.02 series, we find that the 0.09 < x < 0.3 composition region, where superconductivity is suppressed, has large
We have investigated the specific heat of optimally-doped iron chalcogenide superconductor Fe(Te 0.57 Se 0.43 ) with a high-quality single crystal sample. The electronic specific heat C e of this sample has been successfully separated from the phonon contribution using the specific heat of a non-superconducting sample (Fe 0.90 Cu 0.10 )(Te 0.57 Se 0.43 ) as a reference. The normal state Sommerfeld coefficient n of the superconducting sample is found to be ~ 26.6 mJ/mol K 2 , indicating intermediate electronic correlation. The temperature dependence of e C in the superconducting state can be best fitted using a double-gap model with c 2 (0)/ 3.92 s B k T and c 2 (0)/ 5.84 l B k T . The large gap magnitudes derived from fitting, as well as the large specific heat jump of e c n c ( ) / ~2.11 C T T , indicate strong-coupling superconductivity.Furthermore, the magnetic field dependence of specific heat shows strong evidence for multiband superconductivity.
The nature of metallicity and the level of electronic correlations in the antiferromagnetically ordered parent compounds are two important open issues for the iron-based superconductivity. We perform a temperature-dependent angle-resolved photoemission spectroscopy study of Fe1.02Te, the parent compound for iron chalcogenide superconductors. Deep in the antiferromagnetic state, the spectra exhibit a "peak-dip-hump" line shape associated with two clearly separate branches of dispersion, characteristics of polarons seen in manganites and lightly-doped cuprates. As temperature increases towards the Neel temperature (TN ), we observe a decreasing renormalization of the peak dispersion and a counterintuitive sharpening of the hump linewidth, suggestive of an intimate connection between the weakening electron-phonon (e-ph) coupling and antiferromagnetism. Our finding points to the highly-correlated nature of Fe1.02Te ground state featured by strong interactions among the charge, spin and lattice and a good metallicity plausibly contributed by the coherent polaron motion. The role of many-body interactions is one of the central questions for unconventional superconductivity. For the recently discovered iron-based superconductors, the strength of electronic correlations is still an unsettled issue [1,2]. For one of them, iron chalcogenides, a strong correlation scenario has been proposed by theory [3,4] and supported by experiments [5][6][7][8][9][10][11][12]. For their parent compound Fe 1+y Te, while the high-temperature paramagnetic (PM) state shows similar signs for localized physics as in the undoped high-Tc cuprates in transport [11] and optical [12] experiments, the metallic behavior in the low-temperature antiferromagnetic (AFM) state (at T
Superconductors with a chiral p-wave pairing are of great interest because they could support Majorana modes that could enable the development of topological quantum computing technologies that are robust against decoherence. Sr 2 RuO 4 is widely believed to be a chiral p-wave superconductor. Yet, the mechanism by which superconductivity emerges in this, and indeed most other unconventional superconductors, remains unclear. Here we show that the local superconducting transition temperature in the vicinity of lattice dislocations in Sr 2 RuO 4 can be up to twice that of its bulk. This is all the more surprising for the fact that disorder is known to easily quench superconductivity in this material. With the help of a phenomenological theory that takes into account the crystalline symmetry near a dislocation and the pairing symmetry of Sr 2 RuO 4 , we predict that a similar enhancement should emerge as a consequence of symmetry reduction in any superconductor with a two-component order parameter.
Odd-parity, spin-triplet superconductor Sr2RuO4 has been found to feature exotic vortex physics including half-flux quanta trapped in a doubly connected sample and the formation of vortex lattices at low fields. The consequences of these vortex states on the low-temperature magnetoresistive behavior of mesoscopic samples of Sr2RuO4 were investigated in this work using ring device fabricated on mechanically exfoliated single crystals of Sr2RuO4 by photolithography and focused ion beam. With the magnetic field applied perpendicular to the in-plane direction, thin-wall rings of Sr2RuO4 were found to exhibit pronounced quantum oscillations with a conventional period of the full-flux quantum even though the unexpectedly large amplitude and the number of oscillations suggest the observation of vortex-flow-dominated magnetoresistance oscillations rather than a conventional Little-Parks effect. For rings with a thick wall, two distinct periods of quantum oscillations were found in high and low field regimes, respectively, which we argue to be associated with the "lock-in" of a vortex lattice in these thick-wall rings. No evidence for half-flux-quantum resistance oscillations were identified in any sample measured so far without the presence of an in-plane field.
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