Abstract:The violation of a Bell inequality is an experimental observation that forces one to abandon a local realistic worldview, namely, one in which physical properties are (probabilistically) defined prior to and independent of measurement and no physical influence can propagate faster than the speed of light. All such experimental violations require additional assumptions depending on their specific construction making them vulnerable to so-called "loopholes." Here, we use photons and high-efficiency superconducting detectors to violate a Bell inequality closing the fair-sampling loophole, i.e. without assuming that the sample of measured photons accurately represents the entire ensemble. Additionally, we demonstrate that our setup can realize one-sided device-independent quantum key distribution on both sides. This represents a significant advance relevant to both fundamental tests and promising quantum applications. Introduction:In 1935, Einstein, Podolsky, and Rosen (EPR) (1) argued that quantum mechanics is incomplete when assuming that no physical influence can be faster than the speed of light and that properties of physical systems are elements of reality. They considered measurements on spatially separated pairs of entangled particles. Measurement on one particle of an entangled pair projects the other instantly on a well-defined state, independent of their spatial separation. In 1964, Bell (2) showed that no local realistic theory can reproduce all quantum mechanical predictions for entangled states. His renowned Bell inequality proved that there is an upper limit to the strength of the observed correlations predicted by local realistic theories. Quantum theory's predictions violate this limit.

Single photons with helical phase structures may carry a quantized amount of orbital angular momentum (OAM), and their entanglement is important for quantum information science and fundamental tests of quantum theory. Because there is no theoretical upper limit on how many quanta of OAM a single photon can carry, it is possible to create entanglement between two particles with an arbitrarily high difference in quantum number. By transferring polarization entanglement to OAM with an interferometric scheme, we generate and verify entanglement between two photons differing by 600 in quantum number. The only restrictive factors toward higher numbers are current technical limitations. We also experimentally demonstrate that the entanglement of very high OAM can improve the sensitivity of angular resolution in remote sensing.