A green organic light-emitting device (OLED) with an extremely high power efficiency of over 100 lm W(-1) is realized through energy transfer from an exciplex. An optimized OLED showed a maximum external efficiency of 25.7%, and a power efficiency of 79.4 lm W(-1) at 1000 cd m(-2) , which is 1.6-times higher than that of state-of-the-art green thermally activated delayed fluorescence (TADF) OLEDs.
Two blue thermally activated delayed fluorescence molecules based on bis(phenylsulfonyl)benzene with very small singlet-triplet splitting energy were designed and synthesized by combining 3,6-di-tert-butylcarbazole with 1,4-bis(phenylsulfonyl)benzene and 1,3-bis(phenylsulfonyl)benzene, and a maximum external quantum efficiency of 11.7% was achieved for an electroluminescent device.
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