We experimentally demonstrate for the first time that a radially polarized field can be focused to a spot size significantly smaller [0.16(1)lambda(2)] than for linear polarization (0.26lambda(2)). The effect of the vector properties of light is shown by a comparison of the focal intensity distribution for radially and azimuthally polarized input fields. For strong focusing, a radially polarized field leads to a longitudinal electric field component at the focus which is sharp and centered at the optical axis. The relative contribution of this component is enhanced by using an annular aperture.

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We demonstrate an experimental method to separately test the optical response of a single sub-wavelength nano-structure to tailored electric and magnetic field distributions in the optical domain. For this purpose a highly focused y-polarized TEM10-mode is used which exhibits spatially separated longitudinal magnetic and transverse electric field patterns. By displacing a single sub-wavelength nano-structure, namely a single split-ring resonator (SRR), in the focal plane, different coupling scenarios can be achieved. It is shown experimentally that the single split-ring resonator tested here responds dominantly as an electric dipole. A much smaller but yet statistically significant magnetic dipole contribution is also measured by investigating the interaction of a single SRR with a magnetic field component perpendicular to the SRR plane (which is equivalent to the curl of the electric field) as well as by analyzing the intensity and polarization distribution of the scattered light with high spatial resolution. The developed experimental setup as well as the measurement techniques presented in this paper are a versatile tool to investigate the optical properties of single sub-wavelength nano-structures.

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Abstract:We experimentally demonstrate for the first time that a linearly polarized beam is focussed to an asymmetric spot when using a high-numerical aperture focussing system. This asymmetry was predicted by Richards and Wolf [Proc. R. Soc. London A 253, 358 (1959)] and can only be measured when a polarization insensitive sensor is placed in the focal region. We used a specially modified photodiode in a knife edge type set up to obtain highly resolved images of the total electric energy density distribution at the focus. The results are in good agreement with the predictions of a vectorial focussing theory.The ability to control and focus light is at the heart of the interdisciplinary field of optics and for many applications an exact knowledge of the structure of the focal field is required. Many areas in optical sciences make use of a tightly focussed light beam such as confocal microscopy [1] and optical data storage [2]. A highly concentrated and well matched field is also a necessary requirement for coupling to small quantum systems [3] and applying light forces to microscopic particles [4]. In the regime of strong focussing the widely used scalar theories are inadequate to describe the focal field. A vectorial focussing theory is required instead. In the concrete example of a beam which is linearly polarized along the y-axis, the rays propagating in the xz-and in the yz-plane, respectively, contribute differently to the focal field (see figures 1(a), (b)). This has two closely related consequences. The effective numerical aperture in the yz-plane is reduced and the focal spot is elongated in the direction of polarization of the input beam because the rays that propagate in this plane do not add up perfectly at the focus. Associated with this elongation, field components in directions orthogonal to the direction of polarization of the input beam arise. These effects are neglected in scalar descriptions [5], which therefore do not predict the correct spot shape and size. All aspects of the field distribution of a tightly focussed linearly polarized light beam have been studied in theory taking into account the vector properties of the field [6,7,8,9]. The theoretical calculations predict pronounced deviations from the results of the scalar theory. Nevertheless, a major part of the intensity 1 is still predicted to be contained in a field 1 In the following, intensity always refers to electric energy density, which is the part of the field energy that couples to standard photodetectors and photosensitive materials. 1Figure 1: Plane wave model for focussing a beam which is linearly polarized parallel to the y-axis. Cross sections for two planes which contain the optical axis, (a) perpendicular and (b) parallel to the direction of polarization, show that the contribution to the total field of the rays propagating under a large angle to the optical axis is weaker in (b). Calculated intensity patterns for the three orthogonal field components (c-e) and total intensity distribution (f). The direction of polariz...