Recent advances in nanomaterials and nano-microfabrication have enabled the development of flexible wearable electronics. However, existing manufacturing methods still rely on a multi-step, error-prone complex process that requires a costly cleanroom facility. Here, we report a new class of additive nanomanufacturing of functional materials that enables a wireless, multilayered, seamlessly interconnected, and flexible hybrid electronic system. All-printed electronics, incorporating machine learning, offers multi-class and versatile human-machine interfaces. One of the key technological advancements is the use of a functionalized conductive graphene with enhanced biocompatibility, anti-oxidation, and solderability, which allows a wireless flexible circuit. The high-aspect ratio graphene offers gel-free, high-fidelity recording of muscle activities. The performance of the printed electronics is demonstrated by using real-time control of external systems via electromyograms. Anatomical study with deep learning-embedded electrophysiology mapping allows for an optimal selection of three channels to capture all finger motions with an accuracy of about 99% for seven classes.

Chiral magnetic domain walls are of great interest because lifting the energetic degeneracy of left-and right-handed spin textures in magnetic domain walls enables fast current-driven domain wall propagation. Although two types of magnetic domain walls are known to exist in magnetic thin films, Bloch-and Néel-walls, up to now the stabilization of homochirality was restricted to Néel-type domain walls. Since the driving mechanism of thin-film magnetic chirality, the interfacial Dzyaloshinskii-Moriya interaction, is thought to vanish in Bloch-type walls, homochiral Bloch walls have remained elusive. Here we use real-space imaging of the spin texture in iron/nickel bilayers on tungsten to show that chiral domain walls of mixed Bloch-type and Néel-type can indeed be stabilized by adding uniaxial strain in the presence of interfacial Dzyaloshinskii-Moriya interaction. Our findings introduce Bloch-type chirality as a new spin texture, which may open up new opportunities to design spin-orbitronics devices.

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Herein, we demonstrate CO2-activated macroscopic graphene architectures with trimodal pore systems that consist of 3D inter-networked macroporosity arising from self-assembly, mesoporosity arising from the intervoids of nanosheets, and microporosity via CO2 activation. The existence of micropores residing in hierarchical structures of trimodal porous graphene frameworks (tGFs) contributes to greatly improve the surface area and pore volume, which are ∼3.8 times greater than typical values of existing 3D macroporous graphene monoliths. As confirmed by the specific capacity, the kinetic parameters, and the regeneration capability for chemical adsorption as well as the specific capacitance, the rate capability, and the cycle stability for electrochemical energy storage, the tGFs have an ideal texture for high performance capacitive materials. Furthermore, the tGFs obtain the structurally and energetically homogeneous surface active sites, which dominantly operate through the π-π interactions for adsorption. Consequently, the ultrahigh capacitance and ultrafast capacitive performance of the tGFs for both chemical and electrochemical adsorptions are attributed to hierarchical trimodal porosity and surface chemistry. These results offer a chemical approach combining self-assembly with conventional activation for the construction of 3D hierarchical structures with multimodal porosity.

Chiral spin textures in ultrathin films, such as skyrmions or chiral domain walls, are believed to offer large performance advantages in the development of novel spintronics technologies. While in-plane magnetized films have been studied extensively as media for current- and field-driven domain wall dynamics with applications in memory or logic devices, the stabilization of chiral spin textures in in-plane magnetized films has remained rare. Here we report a phase of spin structures in an in-plane magnetized ultrathin film system where out-of-plane spin orientations within domain walls are stable. Moreover, while domain walls in in-plane films are generally expected to be non-chiral, we show that right-handed spin rotations are strongly favoured in this system, due to the presence of the interfacial Dzyaloshinskii–Moriya interaction. These results constitute a platform to explore unconventional spin dynamics and topological phenomena that may enable high-performance in-plane spin-orbitronics devices.