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The amplification of spontaneous emission is used to initiate laser action. As the phase of spontaneous emission is random, the phase of the coherent laser emission (the carrier phase) will also be random each time laser action begins. This prevents phase-resolved detection of the laser field. Here, we demonstrate how the carrier phase can be fixed in a semiconductor laser: a quantum cascade laser (QCL). This is performed by injection seeding a QCL with coherent terahertz pulses, which forces laser action to start on a fixed phase. This permits the emitted laser field to be synchronously sampled with a femtosecond laser beam, and measured in the time domain. We observe the phase-resolved buildup of the laser field, which can give insights into the laser dynamics. In addition, as the electric field oscillations are directly measured in the time domain, QCLs can now be used as sources for time-domain spectroscopy.

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Nonlinear couplings between photons and electrons in new materials give rise to a wealth of interesting nonlinear phenomena [1]. This includes frequency mixing, optical rectification or nonlinear current generation, which are of particular interest for generating radiation in spectral regions that are difficult to access, such as the terahertz gap. Owing to its specific linear dispersion and high electron mobility at room temperature, graphene is particularly attractive for realizing strong nonlinear effects [2]. However, since graphene is a centrosymmetric material, second-order nonlinearities a priori cancel, which imposes to rely on less attractive third-order nonlinearities [3]. It was nevertheless recently demonstrated that dc-second-order nonlinear currents [4] as well as ultrafast ac-currents [5] can be generated in graphene under optical excitation. The asymmetry is introduced by the excitation at oblique incidence, resulting in the transfer of photon momentum to the electron system, known as the

The generation of ultrashort pulses from quantum cascade lasers (QCLs) has proved to be challenging. It has been suggested that the ultrafast electron dynamics of these devices is the limiting factor for modelocking and hence pulse formation. Even so, clear modelocking of terahertz (THz) QCLs has been recently demonstrated but the exact mechanism for pulse generation is not fully understood. Here we demonstrate that the dominant factor necessary for active pulse generation is in fact the synchronization between the propagating electronic modulation and the generated THz pulse in the QCL. By using phase resolved detection of the electric field in QCLs embedded in metal-metal waveguides, we demonstrate that active modelocking requires the phase velocity of the microwave round trip modulation to equal the group velocity of the THz pulse. This allows the THz pulse to propagate in phase with the microwave modulation along the gain medium, permitting short pulse generation. Modelocking was performed on QCLs employing phonon depopulation active regions, permitting coherent detection of large gain bandwidths (500 GHz), and the generation of 11 ps pulses centered around 2.6 THz when the above 'phase-matching' condition is satisfied. This work brings an enhanced understanding of QCL modelocking and will permit new concepts to be explored to generate shorter and more intense pulses from mid-infrared, as well as THz, QCLs.

International audienceDispersion compensation is vital for the generation of ultrashort and single cycle pulses from modelocked lasers across the electromagnetic spectrum. It is typically based on addition of an extra dispersive element to the laser cavity that introduces a chromatic dispersion opposite to that of the gain medium. To date, however, no dispersion compensation schemes have been successfully applied to terahertz (THz) quantum cascade lasers for short and stable pulse generation in the THz range. In this work, a monolithic on-chip compensation scheme is realized for a modelocked QCL, permitting THz pulses to be considerably shortened from 16ps to 4ps. This is based on the realization of a small coupled cavity resonator that acts as an 'off resonance' Gires-Tournois interferometer (GTI), permitting large THz spectral bandwidths to be compensated. This novel application of a GTI opens up a direct and simple route to sub-picosecond and single cycle pulses in the THz range from a compact semiconductor source

By directly modulating the bias voltage of a double-metal waveguide, 2.8THz quantum cascade laser, we observe the appearance of multiple gigahertz sidebands in the emission spectrum, with a spacing that can be continuously tuned up to 13GHz. By using an upconversion technique, the terahertz spectrum is shifted at 1.57μm, and displayed on an optical spectrum analyzer. A marked increase in the number of sidebands is observed when the modulation frequency approaches the round-trip frequency (∼12.3GHz). The laser packaging high frequency response has been measured using a microwave rectification technique, and is limited by the bond-wire parasitic inductance.

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