In a planar organic light-emitting diode (OLED), over 50% of emitted lights are trapped as a waveguide mode in the organic-indium tin oxide layer and as a surface plasmon polariton mode at the metal and organic layer interface. The light extraction efficiency into the glass substrate is greatly enhanced when the organic/Al interface of the OLED is patterned with a graded photonic super-crystal (GPSC), by destroying the plasmonic resonance condition through graded patterns and by scattering the surface plasmon polariton into the glass. The light extraction efficiency increases with the area fraction of graded regions in the GPSC. The efficiency can reach above 68.5%, 72.9%, and 78.9% for octagonal, square, and triangular GPSCs with area fractions of the graded regions of 53.9%, 78.5%, and 90.7%, respectively. The light extraction efficiency goes up to 83.0%, 81.2%, and 79.0% at the wavelengths of 447, 507, and 608 nm, respectively, in OLED patterned with triangular GPSC, compared with the targeted efficiency of 70%.

Twistronics has been studied for manipulating electronic properties through a twist angle in the formed moiré superlattices of two dimensional layer materials. In this paper, we study twistoptics for manipulating optical properties in twisted moiré photonic patterns without physical rotations. We describe a theoretic approach for the formation of single-layer twisted photonic pattern in square and triangular lattices through an interference of two sets of laser beams arranged in two cone geometries. The moiré period and the size of unit super-cell of moiré patterns are related to the twist angle that is calculated from the wavevector ratio of laser beams. The bright and dark regions in moiré photonic pattern in triangular lattices are reversible. We simulate E-field intensities and their cavity quality factors for resonance modes in moiré photonic pattern in square lattices. Due to the bandgap dislocation between the bright and dark regions, the resonance modes with very high quality-factors appears near bandgap edges for the moiré photonic pattern with a twist angle of 9.5 degrees. At the low frequency range, the resonance modes can be explained as Mie resonances. The cavity quality factor decreases for resonance modes when the twist angle is increased to 22.6 degrees.

The study of twisted bilayer 2D materials has revealed many interesting physics properties. A twisted moiré photonic crystal is an optical analog of twisted bilayer 2D materials. The optical properties in twisted photonic crystals have not yet been fully elucidated. In this paper, we generate 2D twisted moiré photonic crystals without physical rotation and simulate their photonic band gaps in photonic crystals formed at different twisted angles, different gradient levels, and different dielectric filling factors. At certain gradient levels, interface modes appear within the photonic band gap. The simulation reveals “tic tac toe”-like and “traffic circle”-like modes as well as ring resonance modes. These interesting discoveries in 2D twisted moiré photonic crystal may lead toward its application in integrated photonics.

The layer edge states or low energy state (LES) in 2D hybrid organic–inorganic perovskites demonstrate a prolonged carrier lifetime for better performance of optoelectronic devices. However, the fundamental understanding of LES in 2D perovskites is still inconclusive. Herein, a photoluminescence (PL) study of LES in 2D Ruddlesden–Popper perovskites is presented with n = 2 and n = 3 from their cleaved cross sections that are more stable than the natural edge. The PL measurements clearly observe reversible, and irreversible surface relaxations (case I and case II) in three laser intensity ranges, further supported by a PL excitation cycle from low to high laser intensity, and vice versa. The PL wavelength of LES is tunable with laser intensity and blueshifts with increasing laser intensity during irreversible surface relaxation process (case I). Fluorescence lifetime imaging (FLIM) shows that the LES has a longer lifetime than the band‐edge emission in the sample without a photodegradation, while the BE lifetime becomes relatively longer in the area with a photodegradation. The presented laser tunable LES and the related irreversible relaxation process provide a new insight that can help improve the photostability in 2D perovskites and understand roles of LESs in optoelectronic device performance.

A moiré photonic crystal is an optical analog of twisted graphene. A 3D moiré photonic crystal is a new nano-/microstructure that is distinguished from bilayer twisted photonic crystals. Holographic fabrication of a 3D moiré photonic crystal is very difficult due to the coexistence of the bright and dark regions, where the exposure threshold is suitable for one region but not for the other. In this paper, we study the holographic fabrication of 3D moiré photonic crystals using an integrated system of a single reflective optical element (ROE) and a spatial light modulator (SLM) where nine beams (four inner beams + four outer beams + central beam) are overlapped. By modifying the phase and amplitude of the interfering beams, the interference patterns of 3D moiré photonic crystals are systemically simulated and compared with the holographic structures to gain a comprehensive understanding of SLM-based holographic fabrication. We report the holographic fabrication of phase and beam intensity ratio-dependent 3D moiré photonic crystals and their structural characterization. Superlattices modulated in the z-direction of 3D moiré photonic crystals have been discovered. This comprehensive study provides guidance for future pixel-by-pixel phase engineering in SLM for complex holographic structures.

It is challenging to realize the complete broadband absorption of near-infrared in thin optical devices. In this paper, we studied high light absorption in two devices: a stack of Au-pattern/insulator/Au-film and a stack of Au-pattern/weakly-absorbing-material/Au-film where the Au-pattern was structured in graded photonic super-crystal. We observed multiple-band absorption, including one near 1500 nm, in a stack of Au-pattern/spacer/Au-film. The multiple-band absorption is due to the gap surface plasmon polariton when the spacer thickness is less than 30 nm. Broadband absorption appears in the near-infrared when the insulator spacer is replaced by a weakly absorbing material. E-field intensity was simulated and confirmed the formation of gap surface plasmon polaritons and their coupling with Fabry–Pérot resonance.

The laser diffraction from periodic structures typically shows isolated and sharp point patterns at zeroth and ±nth orders. Diffraction from 2D graded photonic super-crystals (GPSCs) has demonstrated over 1000 spots due to the fractional diffractions. Here, we report the holographic fabrication of three types of 3D GPSCs through nine beam interferences and their characteristic diffraction patterns. The diffraction spots due to the fractional orders are merged into large-area diffraction zones for these three types of GPSCs. Three distinguishable diffraction patterns have been observed: (a) 3 × 3 Diffraction zones for GPSCs with a weak gradient in unit super-cell, (b) 5 × 5 non-uniform diffraction zones for GPSCs with a strong modulation in long period and a strong gradient in unit super-cell, (c) more than 5 × 5 uniform diffraction zones for GPSCs with a medium gradient in unit super-cell and a medium modulation in long period. The GPSCs with a strong modulation appear as moiré photonic crystals. The diffraction zone pattern not only demonstrates a characterization method for the fabricated 3D GPSCs, but also proves their unique optical properties of the coupling of light from zones with 360° azimuthal angles and broad zenith angles.