Cavity quantum electrodynamics, a central research field in optics and solid-state physics, addresses properties of atom-like emitters in cavities and can be divided into a weak and a strong coupling regime. For weak coupling, the spontaneous emission can be enhanced or reduced compared with its vacuum level by tuning discrete cavity modes in and out of resonance with the emitter. However, the most striking change of emission properties occurs when the conditions for strong coupling are fulfilled. In this case there is a change from the usual irreversible spontaneous emission to a reversible exchange of energy between the emitter and the cavity mode. This coherent coupling may provide a basis for future applications in quantum information processing or schemes for coherent control. Until now, strong coupling of individual two-level systems has been observed only for atoms in large cavities. Here we report the observation of strong coupling of a single two-level solid-state system with a photon, as realized by a single quantum dot in a semiconductor microcavity. The strong coupling is manifest in photoluminescence data that display anti-crossings between the quantum dot exciton and cavity-mode dispersion relations, characterized by a vacuum Rabi splitting of about 140 microeV.
Conventional semiconductor laser emission relies on stimulated emission of photons, which sets stringent requirements on the minimum amount of energy necessary for its operation. In comparison, exciton-polaritons in strongly coupled quantum well microcavities can undergo stimulated scattering that promises more energy-efficient generation of coherent light by 'polariton lasers'. Polariton laser operation has been demonstrated in optically pumped semiconductor microcavities at temperatures up to room temperature, and such lasers can outperform their weak-coupling counterparts in that they have a lower threshold density. Even though polariton diodes have been realized, electrically pumped polariton laser operation, which is essential for practical applications, has not been achieved until now. Here we present an electrically pumped polariton laser based on a microcavity containing multiple quantum wells. To prove polariton laser emission unambiguously, we apply a magnetic field and probe the hybrid light-matter nature of the polaritons. Our results represent an important step towards the practical implementation of polaritonic light sources and electrically injected condensates, and can be extended to room-temperature operation using wide-bandgap materials.
We observe antibunching in the photons emitted from a strongly-coupled single quantum dot and pillar microcavity in resonance. When the quantum dot was spectrally detuned from the cavity mode, the cavity emission remained antibunched, and also anticorrelated from the quantum dot emission. Resonant pumping of the selected quantum dot via an excited state enabled these observations by eliminating the background emitters that are usually coupled to the cavity. This device demonstrates an on-demand single photon source operating in the strong coupling regime, with a Purcell factor of 61 ± 7 and quantum efficiency of 97%.PACS numbers: 78.67. Hc, 78.55.Cr, 78.90.+t Cavity quantum electrodynamics (CQED), addressing the interaction between a quantum emitter and a cavity, has been a central topic in atomic physics for decades [1,2,3,4] and has recently come to the forefront of semiconductor physics [5,6,7,8]. If the coupling between the single quantum emitter and cavity mode is strong compared to their decay rates, the emitter and cavity coherently exchange energy back and forth leading to Rabi oscillations. This strong coupling (SC) regime is of great interest for a variety of quantum information applications, especially with a solid-state implementation. A SC QD-microcavity system could lead to a nearly ideal single photon source (SPS) for quantum information processing, with extremely high efficiency and photon indistinguishability [9]. The same technology could be applied as an interface between a spin qubit and single photon qubit in a quantum network [10].SC between a single atom and a cavity was first achieved more than a decade ago [4]. An analogous system in the solid-state is the excitonic transition of a semiconductor quantum dot (QD) together with a semiconductor microcavity. Several groups have recently reported SC between a single (In,Ga)As QD and either micropillar [5], photonic crystal [6], or microdisk [7] resonators. SC can also occur between a single cavity mode and a collection of degenerate emitters, such as an ensemble of atoms or a quantum well [11]. However, in the latter case the behavior is classical: adding or removing one emitter or one photon from the system has little effect.In previous studies of QD-cavity SC [5,6,7] it was argued that the spectral density of QDs was sufficiently low that it is unlikely that several degenerate emitters contributed to the anticrossing. However, it was not verified that the system had one and only one emitter. There was a surprisingly large amount of emission from the cavity mode when the QD was far detuned. It was unclear whether this emission originated from the particular single QD or from many background emitters. An important step to establish SC in solid-state CQED is verification that the double-peaked spectrum originates from a single quantum emitter, not a collection of emitters, interacting with the cavity mode.In this Letter we present proof that the emission from a strongly-coupled QD-microcavity system is dominated by a single quantum emitter....
We present measurements of first- and second-order coherence of quantum-dot micropillar lasers together with a semiconductor laser theory. Our results show a broad threshold region for the observed high-beta microcavities. The intensity jump is accompanied by both pronounced photon intensity fluctuations and strong coherence length changes. The investigations clearly visualize a smooth transition from spontaneous to predominantly stimulated emission which becomes harder to determine for high beta. In our theory, a microscopic approach is used to incorporate the semiconductor nature of quantum dots. The results are in agreement with the experimental intensity traces and the photon statistics measurements.
The authors report on AlAs∕GaAs micropillar cavities with unprecedented quality factors based on high reflectivity distributed Bragg reflectors (DBRs). Due to an increased number of mirror pairs in the DBRs and an optimized etching process record quality (Q) factors up to 165.000 are observed for micropillars with diameters of 4μm. Optical studies reveal a very small ellipticity of 5×10−4 of the pillar cross section. Because of the high Q factors, strong coupling with a vacuum Rabi splitting of 23μeV is observed for micropillars with a diameter of 3μm.
We probe the indistinguishability of photons emitted by a semiconductor quantum dot (QD) via time- and temperature-dependent two-photon interference (TPI) experiments. An increase in temporal separation between consecutive photon emission events reveals a decrease in TPI visibility on a nanosecond time scale, theoretically described by a non-Markovian noise process in agreement with fluctuating charge traps in the QD's vicinity. Phonon-induced pure dephasing results in a decrease in TPI visibility from (96±4)% at 10 K to a vanishing visibility at 40 K. In contrast to Michelson-type measurements, our experiments provide direct access to the time-dependent coherence of a quantum emitter on a nanosecond time scale.
The success of advanced quantum communication relies crucially on non-classical light sources emitting single indistinguishable photons at high flux rates and purity. We report on deterministically fabricated microlenses with single quantum dots inside which fulfil these requirements in a flexible and robust quantum device approach. In our concept we combine cathodoluminescence spectroscopy with advanced in situ three-dimensional electron-beam lithography at cryogenic temperatures to pattern monolithic microlenses precisely aligned to pre-selected single quantum dots above a distributed Bragg reflector. We demonstrate that the resulting deterministic quantum-dot microlenses enhance the photon-extraction efficiency to (23±3)%. Furthermore we prove that such microlenses assure close to pure emission of triggered single photons with a high degree of photon indistinguishability up to (80±7)% at saturation. As a unique feature, both single-photon purity and photon indistinguishability are preserved at high excitation power and pulsed excitation, even above saturation of the quantum emitter.
scite is a Brooklyn-based organization that helps researchers better discover and understand research articles through Smart Citations–citations that display the context of the citation and describe whether the article provides supporting or contrasting evidence. scite is used by students and researchers from around the world and is funded in part by the National Science Foundation and the National Institute on Drug Abuse of the National Institutes of Health.
hi@scite.ai
10624 S. Eastern Ave., Ste. A-614
Henderson, NV 89052, USA
Copyright © 2024 scite LLC. All rights reserved.
Made with 💙 for researchers
Part of the Research Solutions Family.