Organic semiconductor distributed feedback (DFB) lasers are of interest as external or chip-integrated excitation sources in the visible spectral range for miniaturized Raman-on-chip biomolecular detection systems. However, the inherently limited excitation power of such lasers as well as oftentimes low analyte concentrations requires efficient Raman detection schemes. We present an approach using surface-enhanced Raman scattering (SERS) substrates, which has the potential to significantly improve the sensitivity of on-chip Raman detection systems. Instead of lithographically fabricated Au/Ag-coated periodic nanostructures on Si/SiO2 wafers, which can provide large SERS enhancements but are expensive and time-consuming to fabricate, we use low-cost and large-area SERS substrates made via laser-assisted nanoreplication. These substrates comprise gold-coated cyclic olefin copolymer (COC) nanopillar arrays, which show an estimated SERS enhancement factor of up to ∼ 10(7). The effect of the nanopillar diameter (60-260 nm) and interpillar spacing (10-190 nm) on the local electromagnetic field enhancement is studied by finite-difference-time-domain (FDTD) modeling. The favorable SERS detection capability of this setup is verified by using rhodamine 6G and adenosine as analytes and an organic semiconductor DFB laser with an emission wavelength of 631.4 nm as the external fiber-coupled excitation source.
We report on a CEP-stable OPCPA system reaching multi-GW peak powers at 300 kHz repetition rate. It delivers 15 W of average power, over 50 µJ of compressed pulse energy and a pulse duration below 6 fs. By implementing an additional pump-seed-synchronization, the output parameters are stabilized over hours with power fluctuations of less than 1.5%.
We present a 300 W picosecond thin-disk based pump laser designed for amplifying few-cycle pulses by means of optical parametric amplification (OPA). Output energies up to 30 mJ are demonstrated at 10 kHz with a pulse duration of 1.6 ps.
Short-pulse-pumped optical parametric chirped pulse amplification (OPCPA) requires a precise temporal overlap of the interacting pulses in the nonlinear crystal to achieve stable performance. We present active synchronization of the ps-pump pulses and the broadband seed pulses used in an OPCPA system with a residual timing jitter below 2 fs. This unprecedented stability was achieved utilizing optical parametric amplification to generate the error signal, requiring less than 4 pJ of seed- and 10 µJ of pump-pulse-energy in the optical setup. The synchronization system shows excellent long-term performance and can be easily implemented in almost any OPCPA system.
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