Plasmonic nanostructures can overcome Abbe's diffraction limit to generate strong gradient fields, enabling efficient optical trapping of nano-sized particles. However, it remains challenging to achieve stable trapping with low incident laser intensity. Here, we demonstrate a Fano resonance-assisted plasmonic optical tweezers (FAPOT), for single nanoparticle trapping in an array of asymmetrical split nano-apertures, milled on a 50 nm gold thin film. Stable trapping is achieved by tuning the trapping wavelength and varying the incident trapping laser intensity. A very large normalized trap stiffness of 8.65 fN/nm/mW for 20 nm polystyrene particles at a near-resonance trapping wavelength of 930 nm was achieved. We show that trap stiffness on resonance is enhanced by a factor of 63 compared to off-resonance conditions. This can be attributed to the ultra-small mode volume, which enables large near-field strengths and a cavity Purcell effect contribution. These results should facilitate strong trapping with low incident trapping laser intensity, thereby providing new options for studying transition paths of single molecules, such as proteins, DNA, or viruses.

The ability of metallic nanostructures to confine light at the sub-wavelength scale enables new perspectives and opportunities in the field of nanotechnology. Making use of this unique advantage, nano-optical trapping techniques have been developed to tackle new challenges in a wide range of areas from biology to quantum optics. In this work, starting from basic theories, we present a review of research progress in near-field optical manipulation techniques based on metallic nanostructures, with an emphasis on some of the most promising advances in molecular technology, such as the precise control of single biomolecules. We also provide an overview of possible future research directions of nanomanipulation techniques.

The term whispering gallery modes (WGMs) was first introduced to describe the curvilinear propagation of sound waves under a cathedral dome. The physical concept has now been generalized to include light waves that are continuously reflected along the closed concave surface of an optical cavity such as a glass microsphere. The circular path of the internally reflected light results in constructive interference and optical resonance, a morphology-dependent resonance that is suitable for interferometric sensing. WGM resonators are miniature micro-interferometers that use the multiple-cavity passes of light for very sensitive measurements at the micro-and nanoscale, including single molecules and ions measurements. This Primer introduces various WGM sensors based on glass microspheres, microtoroids, microcapillaries and silicon microrings. We describe the sensing mechanisms including mode splitting and resonance shift, exceptional-point-enhanced sensing, and optomechanical and optoplasmonic signal transductions. Applications and experimental results cover in-vivo and single-molecule sensing, gyroscopes and microcavity quantum electrodynamics. Data analysis methods and limitations of the WGM techniques are also discussed.Finally, we provide an outlook for molecule, in-vivo and quantum sensing.

Optical nanofiber waveguides are widely used for near-field delivery and measurement of light. Despite their versatility and efficiency, nanofibers have a critical drawback -their inability to maintain light's polarization state on propagation. Here, we design a directional coupler consisting of two crossed nanofibers to probe the polarization state at the waist region. Directionality of coupling occurs due to asymmetric dipolar emission or spin-locking when the evanescent field pattern breaks the mirror symmetry of the crossed-nanofiber system. We demonstrate that, by monitoring the outputs from the directional coupler, two non-orthogonal polarization states can be prepared at the nanofiber waist with a fidelity higher than 99%. Based on these states, we devise a simple and reliable method for complete control of the polarization along a nanofiber waveguide.

Light guided by an optical nanofibre can have a very steep evanescent field gradient extending from the fibre surface. This can be exploited to drive electric quadrupole transitions in nearby quantum emitters. In this paper, we report on the observation of the 5S 1/2 → 4D 3/2 electric quadrupole transition at 516.6 nm (in vacuum) in laser-cooled 87 Rb atoms using only a few µW of laser power propagating through an optical nanofibre embedded in the atom cloud. This work extends the range of applications for optical nanofibres in atomic physics to include more fundamental tests.

We experimentally demonstrate orbiting of isotropic, dielectric microparticles around an optical nanofiber that guides elliptically polarized fundamental modes. The driving transverse radiation force appears in the evanescent electromagnetic fields due to orbital angular momentum. The force direction is opposite to that of the energy flow circulation around the nanofiber. Our results verify the theoretically predicted negative optical torque on a sufficiently large particle in the vicinity of a nanofiber.

Nanofibre-based optical cavities are particularly useful for quantum optics applications, such as the development of integrated single-photon sources, and for studying fundamental light-matter interactions in cavity quantum electrodynamics (cQED). Although several techniques have been used to produce such cavities, focussed ion beam (FIB) milling is becoming popular; it can be used for the fabrication of complex structures directly in the nanofibre. However, it is challenging to mill insulating materials with highly curved geometries and large aspect ratios, such as silica nanofibres, due to charge accumulation in the material. In this article, we highlight the main features of nanofibres and briefly review cQED with nanofibre-based optical cavities. An overview of the milling process is given with a summary of different FIB milled devices and their applications. Finally, we present our technique to produce nanofibre cavities by FIB milling. To overcome the aforementioned challenges, we present a specially designed base plate with an indium tin oxide (ITO)-coated Si substrate and outline our procedure, which improves stability during milling and increases repeatability.

We report on a controllable, hybrid quantum system consisting of cold Rydberg atoms and an optical nanofiber interface. Using a two-photon ladder-type excitation in 87 Rb, we demonstrate both coherent and incoherent Rydberg excitation at submicron distances from the nanofiber surface. The 780-nm photon, near resonant to the 5S → 5P transition, is mediated by the cooling laser, while the 482-nm light, near resonant to the 5P → 29D transition, is mediated by the guided mode of the nanofiber. The population loss rate of the cold atom ensemble is used to measure the Rydberg population rate. A theoretical model is developed to interpret the results and link the population loss rate to the experimentally measured, effective Rabi frequency of the process. This work makes headway in the study of Rydberg atom-surface interactions at submicron distances and the use of cold Rydberg atoms for all-fibered quantum networks.