Spin caloritronics devices are very important for future development of low-power-consumption technology. We propose a new spin caloritronics device based on zigzag graphene nanoribbon (ZGNR), which is a heterojunction consisting of single-hydrogen-terminated ZGNR (ZGNR-H) and double-hydrogen-terminated ZGNR (ZGNR-H2). We predict that spin-up and spin-down currents flowing in opposite directions can be induced by temperature difference instead of external electrical bias. The thermal spin-up current is considerably large and greatly improved compared with previous work in graphene. Moreover, the thermal colossal magnetoresistance is obtained in our research, which could be used to fabricate highly-efficient spin caloritronics MR devices.
By performing first-principle quantum transport calculations, we studied the transport properties of three kinds of 6,6,12-graphyne nanoribbons with different edges and different cutting directions. The nanoribbon with zigzag edges shows metallic properties and the spin-polarized currents show an obvious negative differential resistance effect, the other two nanoribbons terminated by a phenyl ring are semiconductors and spin-unpolarized. We also designed several nanowire devices based on these 6,6,12-graphyne nanoribbons, such as rectifier, spin filter diode, spin FET and spin caloritronics devices. These results indicate that 6,6,12-graphyne is a potential candidate for spintronics and spin caloritronics.
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