The unique correspondence between mathematical operators and photonic elements in wave optics enables quantitative analysis of light manipulation with individual optical devices. Phase-transition materials are able to provide real-time reconfigurability of these devices, which would create new optical functionalities via (re)compilation of photonic operators, as those achieved in other fields such as field-programmable gate arrays (FPGA). Here, by exploiting the hysteretic phase transition of vanadium dioxide, an all-solid, rewritable metacanvas on which nearly arbitrary photonic devices can be rapidly and repeatedly written and erased is presented. The writing is performed with a low-power laser and the entire process stays below 90 °C. Using the metacanvas, dynamic manipulation of optical waves is demonstrated for light propagation, polarization, and reconstruction. The metacanvas supports physical (re)compilation of photonic operators akin to that of FPGA, opening up possibilities where photonic elements can be field programmed to deliver complex, system-level functionalities.
Solar cells and photocatalysts to yield hydrogen are two significant strategies for taking advantage of clean and sustainable solar energy, and their light manipulation and harvesting ability will play a dominant role in their conversion efficiencies. Butterflies demonstrate their brilliant colors due to their wonderful skills of light manipulation, originating intrinsically from their elaborate architectures. We review the inspiration of butterflies for solar cells and sunlight water-splitting catalysts, focusing on the nipple arrays in butterfly compound eyes, as well as ridge and hole arrays, and the photonic crystal structures in butterfly wing scales. After giving a brief introduction to the typical architectures, we reveal the physical principles lying behind antireflection of compound eyes and black scales and iridescence of wing scales, respective prototypes are extracted and highlighted for the design and fabrication of solar cells and sunlight water-splitting catalysts. We conclude by reviewing the prospects for the integration of these prototypes and the appropriate materials for solar energy, which is the product of an intimate conversation between humanity and nature, as well as close cooperation between scientists from diverse fields.
The recent discovery of ferromagnetism in two-dimensional van der Waals crystals has provoked a surge of interest in the exploration of fundamental spin interaction in reduced dimensions. However, existing material candidates have several limitations, notably lacking intrinsic room-temperature ferromagnetic order and air stability. Here, motivated by the anomalously high Curie temperature observed in bulk diluted magnetic oxides, we demonstrate room-temperature ferromagnetism in Co-doped graphene-like Zinc Oxide, a chemically stable layered material in air, down to single atom thickness. Through the magneto-optic Kerr effect, superconducting quantum interference device and X-ray magnetic circular dichroism measurements, we observe clear evidences of spontaneous magnetization in such exotic material systems at room temperature and above. Transmission electron microscopy and atomic force microscopy results explicitly exclude the existence of metallic Co or cobalt oxides clusters. X-ray characterizations reveal that the substitutional Co atoms form Co2+ states in the graphitic lattice of ZnO. By varying the Co doping level, we observe transitions between paramagnetic, ferromagnetic and less ordered phases due to the interplay between impurity-band-exchange and super-exchange interactions. Our discovery opens another path to 2D ferromagnetism at room temperature with the advantage of exceptional tunability and robustness.
Taking the coupled KdV system as a simple example, analytical and nonsingular
complexiton solutions are firstly discovered in this letter for integrable
systems. Additionally, the analytical and nonsingular positon-negaton
interaction solutions are also firstly found for S-integrable model. The new
analytical positon, negaton and complexiton solutions of the coupled KdV system
are given out both analytically and graphically by means of the iterative
Darboux transformations.Comment: 16 pages, 8 figure
Featuring high photon energy and short wavelength, ultraviolet (UV) light enables numerous applications such as high-resolution imaging, photolithography, and sensing. In order to manipulate UV light, bulky optics are usually required, and hence do not meet the fast-growing requirements of integration in compact systems. Recently, metasurfaces have shown unprecedented control of light, enabling substantial miniaturization of photonic devices from terahertz to visible regions. However, material challenges have hampered the realization of such functionalities at shorter wavelengths. Herein, it is experimentally demonstrated that all-silicon (Si) metasurfaces with thicknesses of only one-tenth of the working wavelength can be designed and fabricated to manipulate broadband UV light with efficiencies comparable to plasmonic metasurface performance in infrared (IR). Also, for the first time, photolithography enabled by metasurface-generated UV holograms is shown. Such performance enhancement is attributed to increased scattering cross sections of Si antennas in the UV range, which is adequately modeled via a circuit. The new platform introduced here will deepen the understanding of light-matter interactions and introduce even more material options to broadband metaphotonic applications, including those in integrated photonics and holographic lithography technologies.
Twist-angle-dependent SHG is observed in noncentrosymmetric twisted bilayer graphene The on-resonance susceptibility is comparable with that of a monolayer MoS 2The nonlinear optical property engineering is achieved by the twisting degree of freedom
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