The tunnel magnetoresistance (TMR) effect in magnetic tunnel junctions (MTJs) is the key to developing magnetoresistive random-access-memory (MRAM), magnetic sensors and novel programmable logic devices. Conventional MTJs with an amorphous aluminium oxide tunnel barrier, which have been extensively studied for device applications, exhibit a magnetoresistance ratio up to 70% at room temperature. This low magnetoresistance seriously limits the feasibility of spintronics devices. Here, we report a giant MR ratio up to 180% at room temperature in single-crystal Fe/MgO/Fe MTJs. The origin of this enormous TMR effect is coherent spin-polarized tunnelling, where the symmetry of electron wave functions plays an important role. Moreover, we observed that their tunnel magnetoresistance oscillates as a function of tunnel barrier thickness, indicating that coherency of wave functions is conserved across the tunnel barrier. The coherent TMR effect is a key to making spintronic devices with novel quantum-mechanical functions, and to developing gigabit-scale MRAM.

There is currently much interest in the development of 'spintronic' devices, in which harnessing the spins of electrons (rather than just their charges) is anticipated to provide new functionalities that go beyond those possible with conventional electronic devices. One widely studied example of an effect that has its roots in the electron's spin degree of freedom is the torque exerted by a spin-polarized electric current on the spin moment of a nanometre-scale magnet. This torque causes the magnetic moment to rotate at potentially useful frequencies. Here we report a very different phenomenon that is also based on the interplay between spin dynamics and spin-dependent transport, and which arises from unusual diode behaviour. We show that the application of a small radio-frequency alternating current to a nanometre-scale magnetic tunnel junction can generate a measurable direct-current (d.c.) voltage across the device when the frequency is resonant with the spin oscillations that arise from the spin-torque effect: at resonance (which can be tuned by an external magnetic field), the structure exhibits different resistance states depending on the direction of the current. This behaviour is markedly different from that of a conventional semiconductor diode, and could form the basis of a nanometre-scale radio-frequency detector in telecommunication circuits.

Neurons in the brain behave as non-linear oscillators, which develop rhythmic activity and interact to process information1. Taking inspiration from this behavior to realize high density, low power neuromorphic computing will require huge numbers of nanoscale non-linear oscillators. Indeed, a simple estimation indicates that, in order to fit a hundred million oscillators organized in a two-dimensional array inside a chip the size of a thumb, their lateral dimensions must be smaller than one micrometer. However, despite multiple theoretical proposals2–5, and several candidates such as memristive6 or superconducting7 oscillators, there is no proof of concept today of neuromorphic computing with nano-oscillators. Indeed, nanoscale devices tend to be noisy and to lack the stability required to process data in a reliable way. Here, we show experimentally that a nanoscale spintronic oscillator8,9 can achieve spoken digit recognition with accuracies similar to state of the art neural networks. We pinpoint the regime of magnetization dynamics leading to highest performance. These results, combined with the exceptional ability of these spintronic oscillators to interact together, their long lifetime, and low energy consumption, open the path to fast, parallel, on-chip computation based on networks of oscillators.

Magnetoresistance (MR) ratio up to 230% at room temperature (294% at 20 K) has been observed in spin-valve-type magnetic tunnel junctions (MTJs) using MgO tunnel barrier layer fabricated on thermally oxidized Si substrates. We found that such a high MR ratio can be obtained when the MgO barrier layer was sandwiched with amorphous CoFeB ferromagnetic electrodes. Microstructure analysis revealed that the MgO layer with (001) fiber texture was realized when the MgO layer was grown on amorphous CoFeB rather than on polycrystalline CoFe. Since there have been no theoretical studies on the MTJs with a crystalline tunnel barrier and amorphous electrodes, the detailed mechanism of the huge tunneling MR effect observed in this study is not clear at the present stage. Nevertheless, the present work is of paramount importance in realizing high-density magnetoresistive random access memory and read head for ultra high-density hard-disk drives into practical use.

When an electric current passes from one ferromagnetic layer via a non-magnetic layer into another ferromagnetic layer, the spin polarization and subsequent rotation of this current can induce a transfer of angular momentum that exerts a torque on the second ferromagnetic layer 1-4 . This provides a potentially useful method to reverse 3,5-7 and oscillate 8 the magnetic momenta in nanoscale magnetic structures. Owing to the large current densities required to observe spin-torqueinduced magnetization switching and microwave emission (∼10 7 A cm −2 ), accurately measuring the strength, or even the direction, of the associated spin torque has proved difficult. Yet, such measurements are crucial to refining our understanding of the mechanisms responsible and the theories that describe them 9,10 . To address this, we present quantitative experimental measurements of the spin torque in MgO-based magnetic tunnel junctions 11-14 for a wide range of bias currents covering the switching currents. The results verify the occurrence of two different spin-torque regimes with different bias dependences that agree well with theoretical predictions 10 .Magnetic tunnel junctions (MTJs) consisting of a MgO insulating layer sandwiched between two ferromagnetic layers (S 1 and S 2 in Fig. 1a) were used to provide very large magnetoresistance 11,14 . Such MTJs are now useful as data storage cells in magnetic random-access memories (M-RAMs) and as magnetic-field sensors in magnetic hard disk drives [11][12][13] . The MTJs with a layer structure of Ir-Mn/Co-Fe/Ru/Co 60 Fe 20 B 20 /MgO/Co 60 Fe 20 B 20 were prepared on a MgO substrate using an ultrahigh-vacuum sputtering system (C-7100; Canon ANELVA). The 3-nm-thick bottom Co-Fe-B layer (S 1 ) acts as a spin polarizer. The top Co-Fe-B layer (S 2 ), a 2-nm-thick free layer, is excited by the spin torque. The MgO tunnel barrier is about 1 nm thick. The MTJs are rectangular with dimensions of approximately 70 nm × 250 nm (see the Methods section for preparation details).Resistance-magnetic-field (R-H ) curves measured at a small bias voltage (0.1-0.3 mV) and different in-plane field directions, that is, θ H = 0 and 45 • , are shown in Fig. 1b. θ H is the angle between the applied field direction and the easy axis of the magnetic cell along the long axis of the rectangular cell (see Fig. 1a). The magnetoresistance ratio is defined as MR = (R AP − R P )/R P , where R P and R AP respectively represent resistance in the parallel and antiparallel magnetization alignments of S 1 and S 2 . A positive bias current denotes electron flow from S 2 to S 1 . The magnetoresistance ratio and R P at a small bias voltage are, respectively, 154% and about 120 (R P × (Junction area) = 2 µm 2 ). Figure 1c shows the bias voltage, V b , dependence of the tunnelling resistance, as measured in four different fields (A-D), which are indicated by arrows in Fig. 1b. For antiparallel alignment (curves A and B), the resistance decreases with increasing V b because new tunnelling channels open at higher bias voltages 1...

A magnetic tunnel junction (MTJ), which consists of a thin insulating layer (a tunnel barrier) sandwiched between two ferromagnetic electrode layers, exhibits tunnel magnetoresistance (TMR) due to spin-dependent electron tunnelling. Since the 1995 discovery of room-temperature TMR, MTJs with an amorphous aluminium oxide (Al–O) tunnel barrier have been studied extensively. Al–O-based MTJs exhibit magnetoresistance (MR) ratios up to about 70% at room temperature (RT) and are currently used in magnetoresistive random access memory (MRAM) and the read heads of hard disk drives. MTJs with MR ratios significantly higher than 70% at RT, however, are needed for next-generation spintronic devices. In 2001 first-principle theories predicted that the MR ratios of epitaxial Fe/MgO/Fe MTJs with a crystalline MgO(0 0 1) barrier would be over 1000% because of the coherent tunnelling of fully spin-polarized Δ1 electrons. In 2004 MR ratios of about 200% were obtained in MTJs with a single-crystal MgO(0 0 1) barrier or a textured MgO(0 0 1) barrier. CoFeB/MgO/CoFeB MTJs for practical applications were also developed and found to have MR ratios up to 500% at RT. MgO-based MTJs are of great importance not only for device applications but also for clarifying the physics of spin-dependent tunnelling. In this article we introduce recent studies on physics and applications of the giant TMR in MgO-based MTJs.

Spin-momentum transfer between a spin-polarized current and a ferromagnetic layer can induce steady-state magnetization precession, and has recently beenproposed as a working principle for ubiquitous radio-frequency devices for radar and telecommunication applications. However, to-date, the development of industrially attractive prototypes has been hampered by the inability to identify systems which can provide enough power. Here, we demonstrate that microwave signals with device-compatible output power levels can be generated from a single magnetic tunnel junction with a lateral size of 100 nm, seven orders of magnitude smaller than conventional radio-frequency oscillators. We find that in MgO magnetic tunnel junctions the perpendicular torque induced by the spin-polarized current on the local magnetization can reach 25% of the in-plane spin-torque term, while exhibiting a different bias-dependence. Both findings contrast with the results obtained on all-metallic structures -previously investigated -, reflecting the fundamentally different transport mechanisms in the two types of structures.Mizuguchi for discussions.

Spin-polarized current can excite the magnetization of a ferromagnet through the transfer of spin angular momentum to the local spin system. This pure spin-related transport phenomenon leads to alluring possibilities for the achievement of a nanometer scale, complementary metal oxide semiconductor-compatible, tunable microwave generator that operates at low bias for future wireless communication applications. Microwave emission generated by the persistent motion of magnetic vortices induced by a spin-transfer effect seems to be a unique manner to reach appropriate spectral linewidth. However, in metallic systems, in which such vortex oscillations have been observed, the resulting microwave power is much too small. In this study, we present experimental evidence of spin-transfer-induced vortex precession in MgObased magnetic tunnel junctions, with an emitted power that is at least one order of magnitude stronger and with similar spectral quality. More importantly and in contrast to other spintransfer excitations, the thorough comparison between experimental results and analytical predictions provides a clear textbook illustration of the mechanism of spin-transfer-induced vortex precession.