Stretchable conductor is one of the key components in soft electronics that allows seamless integration of electronic devices and sensors on elastic substrates. Its unique advantages of mechanical flexibility and stretchability have enabled a variety of wearable bioelectronic devices that can conformably adapt to curved skin surface for long-term health monitoring applications. Here, we report a poly(3,4ethylenedioxythiophene) polystyrene sulfonate (PEDOT:PSS)-based stretchable polymer blend that can be patterned using an inkjet printing process while exhibiting low sheet resistance and accommodating large mechanical deformations. We have systematically studied the effect of various types of polar solvent additives that can help induce phase separation of PEDOT and PSS grains and changes the conformation of PEDOT chain thereby improving the electrical property of the film by facilitating charge hopping along the percolating PEDOT network. The optimal ink formulation is achieved by adding 5 wt% of ethylene glycol into pristine PEDOT:PSS aqueous solution which results in a sheet resistance of as low as 58 Ω/ .Elasticity can also be achieved by blending the above solution with soft polymer poly(ethylene oxide)
Soft wearable sensors are essential components for applications such as motion tracking, humanmachine interface, and soft robots. However, most of the reported sensors are either specifically designed to target an individual stimulus or capable of responding to multiple stimuli (e.g., pressure and strain) but without the necessary selectivity to distinguish those stimuli. Here we report an elastomeric sponge-based sensor that can respond to and distinguish three different kinds of stimuli: pressure, strain, and temperature. The sensor utilizes a porous polydimethylsiloxane (PDMS) sponge fabricated from a sugar cube sacrificial template, which was subsequently coated with a poly(3,4-ethylenedioxythiophene) polystyrene sulfonate (PEDOT:PSS) conductive polymer through a low-cost dip-coating process. Responses to different types of stimuli can be
Soft electronic devices and sensors have shown great potential for wearable and ambulatory electrophysiologic signal monitoring applications due to their light weight, ability to conform to human skin, and improved wearing comfort, and they may replace the conventional rigid electrodes and bulky recording devices widely used nowadays in clinical settings. Herein, we report an elastomeric sponge electrode that offers greatly reduced electrode−skin contact impedance, an improved signal-to-noise ratio (SNR), and is ideally suited for long-term and motion-artifact-tolerant recording of highquality biopotential signals. The sponge electrode utilizes a porous polydimethylsiloxane sponge made from a sacrificial template of sugar cubes, and it is subsequently coated with a poly(3,4-ethylenedioxythiophene) polystyrenesulfonate (PEDOT:PSS) conductive polymer using a simple dip-coating process. The sponge electrode contains numerous micropores that greatly increase the skin−electrode contact area and help lower the contact impedance by a factor of 5.25 or 6.7 compared to planar PEDOT:PSS electrodes or gold-standard Ag/AgCl electrodes, respectively. The lowering of contact impedance resulted in high-quality electrocardiogram (ECG) and electromyogram (EMG) recordings with improved SNR. Furthermore, the porous structure also allows the sponge electrode to hold significantly more conductive gel compared to conventional planar electrodes, thereby allowing them to be used for long recording sessions with minimal signal degradation. The conductive gel absorbed into the micropores also serves as a buffer layer to help mitigate motion artifacts, which is crucial for recording on ambulatory patients. Lastly, to demonstrate its feasibility and potential for clinical usage, we have shown that the sponge electrode can be used to monitor uterine contraction activities from a patient in labor. With its low-cost fabrication, softness, and ability to record high SNR biopotential signals, the sponge electrode is a promising platform for long-term wearable health monitoring applications.
This paper describes the fabrication, characterization and modeling of fundamental logic gates that can be used for designing biosensors with embedded forward error-correction (FEC). The proposed logic gates (AND and OR) are constructed by patterning antibodies at different spatial locations along the substrate of a lateral flow immunosensor assay. The logic gates operate by converting binding events between an antigen and an antibody into a measurable electrical signal using polyaniline nanowires as the transducer. In this study, B. cereus and E. coli have been chosen as model pathogens. The functionality of the AND and OR logic gates has been validated using conductance measurements with different pathogen concentrations. Experimental results show that the change in conductance across the gates can be modeled as a log-linear response with respect to varying pathogen concentration. Equivalent circuits models for AND and OR logic gates have been derived based on measured results.
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