Spinning thermal radiation is a unique phenomenon observed in condensed astronomical objects, including the Wolf-Rayet star EZ-CMa and the red degenerate star G99-47, due to the existence of strong magnetic fields. Here, by designing symmetry-broken metasurfaces, we demonstrate that spinning thermal radiation with a nonvanishing optical helicity can be realized even without applying a magnetic field. We design nonvanishing optical helicity by engineering a dispersionless band that emits omnidirectional spinning thermal radiation, where our design reaches 39% of the fundamental limit. Our results firmly suggest that metasurfaces can impart spin coherence in the incoherent radiation excited by thermal fluctuations. The symmetry-based design strategy also provides a general pathway for controlling thermal radiation in its temporal and spin coherence.
We develop a novel method based on sources and absorbers to examine quantum scattering in finite, nanoscale systems. We show that the Cauchy (mixed) boundary conditions (BCs) are required to put the scattering theory into an action integral formulation. These complex BCs are reduced to simpler Dirichlet BCs by introducing totally absorbing “stealth regions.” Material properties of these enclosing regions are optimized to give decaying solutions so that the scattering amplitudes vanish at the finite boundaries. With the active scattering region now surrounded by absorbers, we construct an “electron antenna” to provide incident waves. The method retains all the physical aspects of the conventional theory while providing new insights into “near-field” scattering effects. The action integral is discretized and evaluated to derive the local wavefunction everywhere. In two-dimensional quantum waveguides, we obtain the scattered wavefunction for geometrically complex scattering centers, showing the flexibility of our method. The modal decomposition of reflected and transmitted waves allows us to obtain transmission coefficients for both propagating and evanescent modes. Using group theory, we develop selection rules for the scattered modes depending on the symmetry of the potential. Our method outperforms the limitations of traditional perturbative estimates, transfer-matrix, S-matrix discretizations, and other schemes to provide a complete nonasymptotic variational description for electron transport in quantum waveguides.
Monolayer transition-metal dichalcogenides (TMDC) have emerged as promising candidates for thermoelectric applications due to their large effective mass and low thermal conductivity. In this article, we study the thermoelectric performance...
Confined geometries such as semiconductor quantum dots are promising candidates for fabricating quantum computing devices. When several quantum dots are in proximity, spatial correlation between electrons in the system becomes significant. In this article, we develop a fully variational action integral formulation for calculating accurate few-electron wavefunctions in configuration space, irrespective of potential geometry. To evaluate the Coulomb integrals with high accuracy, a novel numerical integration method using multiple Gauss quadratures is proposed. Using this approach, we investigate the confinement of two electrons in double quantum dots, and evaluate the spatial entanglement. We investigate the dependence of spatial entanglement on various geometrical parameters. We derive the two-particle wavefunctions in the asymptotic limit of the separation distance between quantum dots, and obtain universal saturation values for the spatial entanglement. Resonances in the entanglement values due to avoided level-crossings of states are observed. We also demonstrate the formation of electron clusters, and show that the entanglement value is a good indicator for the formation of such clusters. Further, we show that a precise tuning of the entanglement values is feasible with applied external electric fields.
Atomistic determination of carrier scattering properties is essential for designing nano-electronic devices in two-dimensional (2D) materials. Traditional quantum scattering theory is developed in an asymptotic limit, thus making it inapplicable for 2D materials and heterostructures. Here, we introduce a new paradigm of non-asymptotic quantum scattering theory to obtain the carrier scattering properties at finite distances from active scattering centers. We develop an atomistic multiscale formalism built on the [Formula: see text] Hamiltonian, supplemented with parameters from first-principles electronic structure calculations. We apply this framework to investigate electron transport in lateral transition-metal dichalcogenide heterostructures and demonstrate enhanced high mobility of the order of [Formula: see text] at room temperature. The non-asymptotic quantum scattering formalism provides a new frontier to design high-performance mesoscopic devices in 2D materials.
Germanium is typically used for solid-state electronics, fiber-optics, and infrared applications, due to its semiconducting behavior at optical and infrared wavelengths. In contrast, here we show that the germanium displays metallic nature and supports propagating surface plasmons in the deep ultraviolet (DUV) wavelengths, that is typically not possible to achieve with conventional plasmonic metals such as gold, silver, and aluminum. We measure the photonic band spectrum and distinguish the plasmonic excitation modes: bulk plasmons, surface plasmons, and Cherenkov radiation using a momentum-resolved electron energy loss spectroscopy. The observed spectrum is validated through the macroscopic electrodynamic electron energy loss theory and first-principles density functional theory calculations. In the DUV regime, intraband transitions of valence electrons dominate over the interband transitions, resulting in the observed highly dispersive surface plasmons. We further employ these surface plasmons in germanium to design a DUV radiation source based on the Smith-Purcell effect. Our work opens a new frontier of DUV plasmonics to enable the development of DUV devices such as metasurfaces, detectors, and light sources based on plasmonic germanium thin films.
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