We illustrate a new method of analyzing three-dimensional momentum images of high-energy photoelectrons generated by intense phase-stabilized few-cycle laser pulses. Using photoelectron momentum spectra that were obtained by velocity-map imaging of above-threshold ionization of xenon and argon targets, we show that the absolute carrier-envelope phase, the laser peak intensity, and pulse duration can be accurately determined simultaneously (with an error of a few percent). We also show that the target structure, in the form of electron-target ion elastic differential cross sections, can be retrieved over a range of energies. The latter offers the promise of using laser-generated electron spectra for probing dynamic changes in molecular targets with subfemtosecond resolution.
Laser-induced electron recollisions are fundamental to many strong field phenomena in atoms and molecules. Using the recently developed quantitative rescattering theory, we demonstrate that the nonsequential double ionization ͑NSDI͒ of atoms by lasers can be obtained quantitatively in terms of inelastic collisions of the target ions with the free returning electrons where the latter are explicitly given by a spectrum-characterized wave packet. Using argon atoms as target, we calculated the NSDI yield including contributions from direct ͑e ,2e͒ electron-impact ionization and electron-impact excitation accompanied by subsequent field ionization. We further investigate the dependence of total NSDI on the carrier-envelope phase of few-cycle laser pulses, and showed that the effect can be experimentally observed by measuring the yield of doubly charged ions only.
Intense (up to a few 10(17) W/ cm2) femtosecond (down to 40 fs) laser pulses are focused onto a partially clusterized argon gas jet. The target was previously characterized and optimized in order to get a homogeneous and dense jet of clusters with a well controlled size. The interaction leads to x-ray emission that is absolutely calibrated and spectrally resolved using a high resolution time-integrated spectrometer in the K-shell range (from 2.9 to 4.3 keV). X-ray spectra are investigated as a function of different laser temporal parameters such as the nanosecond prepulse contrast, the laser pulse duration, and the femtosecond delay between two different laser pulses. The cluster size ranges from 180 to 350 angstroms and irradiation by laser pulses with both linear and circular polarization is investigated. The experimental results are discussed in terms of the laser-cluster interaction dynamics. They are compared with the predictions of collision-dominated nanoplasma models. However, further interaction processes are required in order to explain the observed characteristic lines demonstrating highly charged ions up to Ar16+.
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