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McKeever gives us a comprehensive survey of thermoluminescence, an important, versatile, and widely used experimental technique. Bringing together previously isolated specialized approaches, he stresses the importance of the solid state aspects of the phenomenon. The book contains chapters on analysis and special properties, on instrumentation, and on the variety of defect reaction - using the alkali halides and SiO2 as examples - that can take place within a material to yield thermoluminescence. Three chapters concerning applications discuss the features of the solid state reactions to expain some of the properties observed in practice.
This paper reviews fundamental and practical aspects of optically stimulated luminescence (OSL) dosimetry pertaining to applications in medicine, having particularly in mind new researchers and medical physicists interested in gaining familiarity with the field. A basic phenomenological model for OSL is presented and the key processes affecting the outcome of an OSL measurement are discussed. Practical aspects discussed include stimulation modalities (continuous-wave OSL, pulsed OSL and linear modulation OSL), basic experimental setup, available OSL readers, optical fiber systems and basic properties of available OSL dosimeters. Finally, results from the recent literature on applications of OSL in radiotherapy, radiodiagnostics and heavy charged particle dosimetry are discussed in light of the theoretical and practical framework presented in this review. Open questions and future challenges in OSL dosimetry are highlighted as a guide to the research needed to further advance the field.
The use of thermoluminescence as a method for the dosimetry of ionising radiation has been established for many decades and has been unquestionably successful. It is therefore difficult to imagine how any new technique could easily supplant it. Perhaps optically stimulated luminescence dosimetry should not be characterised as an entirely new technique, but rather a development of the well established technology that may be considered superior in some respects. As is obvious from the tenor of this debate, our two participants are longtime colleagues who have had numerous discussions on this topic. No doubt, many of us will have similar discussions in our own institutions as we weigh the advantages and disadvantages of TLD versus OSL.
Using time-resolved photoluminescence spectroscopy we have measured the lifetime of the F-center luminescence from α-Al2O3:C. The measurements reveal a lifetime of 35–36 ms at room temperature, decreasing to <2 ms over the temperature range from 370 to 500 K. The decrease in the lifetime is shown to follow a classical Mott-Seitz dependence for thermal quenching of luminescence, with an activation energy W of ∼1.08±0.03 eV and a corresponding frequency factor ν of ∼1014 s−1. Similar values for the energy and frequency factor were also obtained from an analysis of thermoluminescence (TL) glow curves measured at different heating rates, when the TL is measured over a wavelength range corresponding to the F-center luminescence emission (centered at 420 nm). Furthermore, the parameters obtained were independent of the glow curve shape, the degree of trap filling, or the specific conditions under which the crystals were grown. This is interpreted as a demonstration that the well-known heating rate dependence of the TL from this material is a result of thermal quenching of the F-center emission. Whereas the thermal quenching parameters obtained from measurement of the luminescence lifetime and from the heating rate analysis of the TL glow curves are independent of the sample type, the degree of trap filling, and the heating or cooling rate, measurements of the photoluminescence intensity, induced by absorption of F-band light, were found to be dependent upon all of the above conditions. This difference in behavior is attributed to a phosphorescence signal from traps associated with the ∼265, ∼310, and ∼450 K TL peaks.
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