Based on the model polyimide systems the principal nonlinear optical features, such as laser induced refractive indices changes, nonlinear refraction and third order susceptibility have been established during their doping with fullerenes, shungites, carbon nanotubes, carbon nanofibers, quantum dots, etc. The evidence of the correlation between laser induced refractive indices and charge carrier mobility has been obtained. The features of new nanocomposites for their possible optoelectronics, laser techniques and solar energy applications have been considered.
Essential improvement of the photorefractive parameters of theorganicstructures has been found via nano- and biostructuring process. The spectral and self-assembling features which can support the photorefractive effect of some conjugated materials, including the liquid crystal ones, have been presented. To investigate the laser-induced change of the refractive index of the nano- and bio-objects-doped materials the holographic recording technique has been used. Moreover some innovative perspective dyes have been applied to study the effect of the rotation of the polarization plane of light. The area of application of the modified materials has been discussed. The tendency to replace the nanotechnology process with the biotechnology ones has been predicted.
Photoconductive and photorefractive characteristics of fullerene- and nanotubes-doped organic thin films based on conjugated organics, such as polyimide, polyaniline, pyridine, etc. have been studied. In addition, the liquid crystal mesophase with nanoobjects has been investigated. The increase of the charge carrier mobility of nanosensitized organics has been established. The nonlinear refraction and cubic nonlinearity have been investigated at wavelength of 532 nm via four-wave mixing technique using Raman-Nath diffraction regime. The thin holographic grating has been written at the spatial frequencies placed in the range of 90-150 mm-1. The energy density has been chosen in the range of 0.1-0.9 J × cm -2. The correlation between photoconductive and nonlinear optical parameters has been revealed. The nanostructured materials can be proposed for different area of nano- and microelectronic applications.
Study and optimization of new nanoscale materials useful for optoelectronic application have been considered. The search for the effective nanostructured materials has been revealed in two directions: to optimize the mechanical hardness of the inorganic systems and to increase the photorefractive parameters of the organics with nanoobjects. It has been testified that the surface mechanical properties of the inorganic materials via nanotubes treatment process can be drastically improved. For example, the surface mechanical hardness of the UV and IR range soft materials can be increased up to 3-10 times under the conditions of oriented nanotubes placement. It has been obtained that the nonlinear optical characteristics (nonlinear refraction n 2 and cubic nonlinearity χ (3) ) of the organics thin films sensitized with fullerenes or nanotubes can be increased up to 3-4 orders of magnitude in comparison with the same parameters for bulk materials traditionally used for nonlinear optics.
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