In this article, we review the history, current status, physical mechanisms,
experimental methods, and applications of nonlinear magneto-optical effects in
atomic vapors. We begin by describing the pioneering work of Macaluso and
Corbino over a century ago on linear magneto-optical effects (in which the
properties of the medium do not depend on the light power) in the vicinity of
atomic resonances, and contrast these effects with various nonlinear
magneto-optical phenomena that have been studied both theoretically and
experimentally since the late 1960s. In recent years, the field of nonlinear
magneto-optics has experienced a revival of interest that has led to a number
of developments, including the observation of ultra-narrow (1-Hz)
magneto-optical resonances, applications in sensitive magnetometry, nonlinear
magneto-optical tomography, and the possibility of a search for parity- and
time-reversal-invariance violation in atoms.Comment: 51 pages, 23 figures, to appear in Rev. Mod. Phys. in Oct. 2002,
Figure added, typos corrected, text edited for clarit
A brief review is given of topics relating to dynamical processes arising in nonlinear interactions between light and resonant systems (atoms or molecules) in the presence of a magnetic field.
The Thirty Meter Telescope (TMT) has been designed to include an adaptive optics system and associated laser guide star (LGS) facility to correct for the image distortion due to Earth's atmospheric turbulence and achieve diffraction-limited imaging. We have calculated the response of mesospheric sodium atoms to a pulsed laser that has been proposed for use in the LGS facility, including modeling of the atomic physics, the light-atom interactions, and the effect of the geomagnetic field and atomic collisions. This particular pulsed-laser format is shown to provide comparable photon return to a continuous-wave (cw) laser of the same average power; both the cw and pulsed lasers have the potential to satisfy the TMT design requirements for photon return flux.
Optical magnetometers measure magnetic fields with extremely high precision and without cryogenics. However, at geomagnetic fields, important for applications from landmine removal to archaeology, they suffer from nonlinear Zeeman splitting, leading to systematic dependence on sensor orientation. We present experimental results on a method of eliminating this systematic error, using the hexadecapole atomic polarization moment. In particular, we demonstrate selective production of the atomic hexadecapole moment at Earth's magnetic field and verify its immunity to nonlinear Zeeman splitting. This technique promises to eliminate directional errors in all-optical atomic magnetometers, potentially improving their measurement accuracy by several orders of magnitude.
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