The ultrafast laser excitation of matters leads to nonequilibrium states with complex solid-liquid phase-transition dynamics. We used electron diffraction at mega-electron volt energies to visualize the ultrafast melting of gold on the atomic scale length. For energy densities approaching the irreversible melting regime, we first observed heterogeneous melting on time scales of 100 to 1000 picoseconds, transitioning to homogeneous melting that occurs catastrophically within 10 to 20 picoseconds at higher energy densities. We showed evidence for the heterogeneous coexistence of solid and liquid. We determined the ion and electron temperature evolution and found superheated conditions. Our results constrain the electron-ion coupling rate, determine the Debye temperature, and reveal the melting sensitivity to nucleation seeds.

A series of Omega experiments have produced and characterized high velocity counter-streaming plasma flows relevant for the creation of collisionless shocks. Single and double CH2 foils have been irradiated with a laser intensity of ∼10 16 W/cm 2 . The laser ablated plasma was characterized 4 mm from the foil surface using Thomson scattering. A peak plasma flow velocity of 2,000 km/s, an electron temperature of ∼110 eV, an ion temperature of ∼30 eV, and a density of ∼10 18 cm −3 were measured in the single foil configuration. Significant increases in electron and ion temperatures were seen in the double foil geometry. The measured single foil plasma conditions were used to calculate the ion skin depth, c/ωpi ∼0.16 mm, the interaction length, int, of ∼8 mm, and the Coulomb mean free path, λ mf p ∼27 mm. With c/ωpi int < λ mf p we are in a regime where collisionless shock formation is possible.

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A laser wakefield acceleration study has been performed in the matched, self-guided, blowout regime producing 720 +/- 50 MeV quasimonoenergetic electrons with a divergence Deltatheta_{FWHM} of 2.85 +/- 0.15 mrad using a 10 J, 60 fs 0.8 microm laser. While maintaining a nearly constant plasma density (3 x 10{18} cm{-3}), the energy gain increased from 75 to 720 MeV when the plasma length was increased from 3 to 8 mm. Absolute charge measurements indicate that self-injection of electrons occurs when the laser power P exceeds 3 times the critical power P{cr} for relativistic self-focusing and saturates around 100 pC for P/P{cr} > 5. The results are compared with both analytical scalings and full 3D particle-in-cell simulations.

We report on the dynamics of ultrafast heating in cryogenic hydrogen initiated by a ≲300  fs, 92 eV free electron laser x-ray burst. The rise of the x-ray scattering amplitude from a second x-ray pulse probes the transition from dense cryogenic molecular hydrogen to a nearly uncorrelated plasmalike structure, indicating an electron-ion equilibration time of ∼0.9  ps. The rise time agrees with radiation hydrodynamics simulations based on a conductivity model for partially ionized plasma that is validated by two-temperature density-functional theory.