We present a comprehensive study of the evolution of the nematic electronic
structure of FeSe using high resolution angle-resolved photoemission
spectroscopy (ARPES), quantum oscillations in the normal state and
elastoresistance measurements. Our high resolution ARPES allows us to track the
Fermi surface deformation from four-fold to two-fold symmetry across the
structural transition at ~87 K which is stabilized as a result of the dramatic
splitting of bands associated with dxz and dyz character. The low temperature
Fermi surface is that a compensated metal consisting of one hole and two
electron bands and is fully determined by combining the knowledge from ARPES
and quantum oscillations. A manifestation of the nematic state is the
significant increase in the nematic susceptibility as approaching the
structural transition that we detect from our elastoresistance measurements on
FeSe. The dramatic changes in electronic structure cannot be explained by the
small lattice effects and, in the absence of magnetic fluctuations above the
structural transition, points clearly towards an electronically driven
transition in FeSe stabilized by orbital-charge ordering.Comment: Latex, 8 pages, 4 figure
Cd3As2 is a candidate three-dimensional Dirac semi-metal which has exceedingly high mobility and nonsaturating linear magnetoresistance that may be relevant for future practical applications. We report magnetotransport and tunnel diode oscillation measurements on Cd3As2, in magnetic fields up to 65 T and temperatures between 1.5 K to 300 K. We find the non-saturating linear magnetoresistance persist up to 65 T and it is likely caused by disorder effects as it scales with the high mobility, rather than directly linked to Fermi surface changes even when approaching the quantum limit. From the observed quantum oscillations, we determine the bulk three-dimensional Fermi surface having signatures of Dirac behaviour with non-trivial Berry's phase shift, very light effective quasiparticle masses and clear deviations from the band-structure predictions. In very high fields we also detect signatures of large Zeeman spin-splitting (g ∼ 16).
We report a high-resolution angle-resolved photo-emission spectroscopy study of the evolution of the electronic structure of FeSe1−xSx single crystals. Isovalent S substitution onto the Se site constitutes a chemical pressure which subtly modifies the electronic structure of FeSe at high temperatures and induces a suppression of the tetragonal-symmetry-breaking structural transition temperature from 87 K to 58 K for x = 0.15. With increasing S substitution, we find smaller splitting between bands with dyz and dxz orbital character and weaker anisotropic distortions of the low temperature Fermi surfaces. These effects evolve systematically as a function of both S substitution and temperature, providing strong evidence that an orbital ordering is the underlying order parameter of the structural transition in FeSe1−xSx. Finally, we detect the small inner hole pocket for x=0.12, which is pushed below the Fermi level in the orbitally-ordered low temperature Fermi surface of FeSe. arXiv:1508.05016v1 [cond-mat.supr-con]
The existence of a nematic phase transition in iron-chalcogenide superconductors poses an intriguing question about its impact on superconductivity. To understand the nature of this unique quantum phase transition, it is essential to study how the electronic structure changes across this transition at low temperatures. Here, we investigate the evolution of the Fermi surfaces and electronic interactions across the nematic phase transition of FeSe 1−x S x using Shubnikov-de Haas oscillations in high magnetic fields up to 45 T in the low temperature regime down to 0.4 K. Most of the Fermi surfaces of FeSe 1−x S x monotonically increase in size except for a prominent low frequency oscillation associated with a small, but highly mobile band, which disappears at the nematic phase boundary near x~0.17, indicative of a topological Lifshitz transition. The quasiparticle masses are larger inside the nematic phase, indicative of a strongly correlated state, but they become suppressed outside it. The experimentally observed changes in the Fermi surface topology, together with the varying degree of electronic correlations, will change the balance of electronic interactions in the multi-band system FeSe 1−x S x and promote different k z-dependent superconducting pairing channels inside and outside the nematic phase.
Magnetoresistivity ρxx and Hall resistivity ρxy in ultra high magnetic fields up to 88 T are measured down to 0.15 K to clarify the multiband electronic structure in high-quality single crystals of superconducting FeSe. At low temperatures and high fields we observe quantum oscillations in both resistivity and Hall effect, confirming the multiband Fermi surface with small volumes. We propose a novel approach to identify the sign of the charge carriers corresponding to a particular cyclotron orbit in a compensated metal from magnetotransport measurements. The observed significant differences in the relative amplitudes of the quantum oscillations between the ρxx and ρxy components, together with the positive sign of the high-field ρxy, reveal that the largest pocket should correspond to the hole band. The low-field magnetotransport data in the normal state suggest that, in addition to one hole and one almost compensated electron bands, the orthorhombic phase of FeSe exhibits an additional tiny electron pocket with a high mobility.
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