The pseudogap is a partial gap in the electronic density of states that opens in the normal (non-superconducting) state of cuprate superconductors and whose origin is a long-standing puzzle. Its connection to the Mott insulator phase at low doping (hole concentration, p) remains ambiguous and its relation to the charge order that reconstructs the Fermi surface at intermediate doping is still unclear. Here we use measurements of the Hall coefficient in magnetic fields up to 88 tesla to show that Fermi-surface reconstruction by charge order in the cuprate YBa2Cu3Oy ends sharply at a critical doping p = 0.16 that is distinctly lower than the pseudogap critical point p* = 0.19 (ref. 11). This shows that the pseudogap and charge order are separate phenomena. We find that the change in carrier density n from n = 1 + p in the conventional metal at high doping (ref. 12) to n = p at low doping (ref. 13) starts at the pseudogap critical point. This shows that the pseudogap and the antiferromagnetic Mott insulator are linked.
The three central phenomena of cuprate superconductors are linked by a common doping p*, where the enigmatic pseudogap phase ends, around which the superconducting phase forms a dome, and at which the resistivity exhibits an anomalous linear dependence on temperature as T → 0 (ref. 1). However, the
We report a combined study of the specific heat and de Haas-van Alphen effect in the iron-pnictide superconductor BaFe2(As(1-x)P(x))2. Our data when combined with results for the magnetic penetration depth give compelling evidence for the existence of a quantum critical point close to x=0.30 which affects the majority of the Fermi surface by enhancing the quasiparticle mass. The results show that the sharp peak in the inverse superfluid density seen in this system results from a strong increase in the quasiparticle mass at the quantum critical point.
The metallic state of the underdoped high-Tc cuprates has remained an enigma: How may seemingly disconnected Fermi surface segments, observed in zero magnetic field as a result of the opening of a partial gap (the pseudogap), possess conventional quasiparticle properties? How do the small Fermi-surface pockets evidenced by the observation of quantum oscillations (QO) emerge as superconductivity is suppressed in high magnetic fields? Such QO, discovered in underdoped YBa2Cu3O6.5 (Y123) and YBa2Cu4O8 (Y124), signify the existence of a conventional Fermi surface (FS). However, due to the complexity of the crystal structures of Y123 and Y124 (CuO2 double-layers, CuO chains, low structural symmetry), it has remained unclear if the QO are specific to this particular family of cuprates. Numerous theoretical proposals have been put forward to explain the route toward QO, including materials-specific scenarios involving CuO chains and scenarios involving the quintessential CuO2 planes. Here we report the observation of QO in underdoped HgBa2CuO4+{\delta} (Hg1201), a model cuprate superconductor with individual CuO2 layers, high tetragonal symmetry, and no CuO chains. This observation proves that QO are a universal property of the underdoped CuO2 planes, and it opens the door to quantitative future studies of the metallic state and of the Fermi-surface reconstruction phenomenon in this structurally simplest cuprate.Comment: 17 pages, 5 figure
The nature of the pseudogap phase of cuprates remains a major puzzle. Although there are indications that this phase breaks various symmetries, there is no consensus on its fundamental nature 1 . Although Fermi-surface 2 , transport 3 and thermodynamic 4 signatures of the pseudogap phase are reminiscent of a transition into a phase with antiferromagnetic order 5,6 , there is no evidence for an associated long-range magnetic order. Here we report measurements of the thermal Hall conductivity κ xy in the normal state of four different cuprates (La 1.6-x Nd 0.4 Sr x CuO 4 , La 1.8-x Eu 0.2 Sr x CuO 4 , La 2-x Sr x CuO 4 , and Bi 2 Sr 2-x La x CuO 6+δ ) and show that a large negative κ xy signal is a property of the pseudogap phase, appearing with the onset of that phase at the critical doping p*. Since it is not due to charge carriersas it persists when the material becomes an insulator, at low doping -or magnons -as it exists in the absence of magnetic order -or phonons -since skew scattering
We use the Nernst effect to delineate the boundary of the pseudogap phase in the temperaturedoping phase diagram of hole-doped cuprate superconductors. New data for the Nernst coefficient ν(T ) of YBa2Cu3Oy (YBCO), La1.8−xEu0.2SrxCuO4 (Eu-LSCO) and La1.6−xNd0.4SrxCuO4 (Nd-LSCO) are presented and compared with previously published data on YBCO, Eu-LSCO, Nd-LSCO, and La2−xSrxCuO4 (LSCO). The temperature Tν at which ν / T deviates from its hightemperature linear behaviour is found to coincide with the temperature at which the resistivity ρ(T ) deviates from its linear-T dependence, which we take as the definition of the pseudogap temperature T -in agreement with the temperature at which the antinodal spectral gap detected in angleresolved photoemission spectroscopy (ARPES) opens. We track T as a function of doping and find that it decreases linearly vs p in all four materials, having the same value in the three LSCObased cuprates, irrespective of their different crystal structures. At low p, T is higher than the onset temperature of the various orders observed in underdoped cuprates, suggesting that these orders are secondary instabilities of the pseudogap phase. A linear extrapolation of T (p) to p = 0 yields T (p → 0) TN(0), the Néel temperature for the onset of antiferromagnetic order at p = 0, suggesting that there is a link between pseudogap and antiferromagnetism. With increasing p, T (p) extrapolates linearly to zero at p pc2, the critical doping below which superconductivity emerges at high doping, suggesting that the conditions which favour pseudogap formation also favour pairing. We also use the Nernst effect to investigate how far superconducting fluctuations extend above the critical temperature Tc, as a function of doping, and find that a narrow fluctuation regime tracks Tc, and not T . This confirms that the pseudogap phase is not a form of precursor superconductivity, and fluctuations in the phase of the superconducting order parameter are not what causes Tc to fall on the underdoped side of the Tc dome.
Nematicity has emerged as a key feature of cuprate superconductors, but its link to other fundamental properties such as superconductivity, charge order and the pseudogap remains unclear. Here we use measurements of transport anisotropy in YBa2Cu3Oy to distinguish two types of nematicity. The first is associated with short-range charge-density-wave modulations in a doping region near p = 0.12. It is detected in the Nernst coefficient, but not in the resistivity. The second type prevails at lower doping, where there are spin modulations but no charge modulations. In this case, the onset of in-plane anisotropy − detected in both the Nernst coefficient and the resistivity − follows a line in the temperature-doping phase diagram that tracks the pseudogap energy. We discuss two possible scenarios for the latter nematicity.
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