Coupling between electrons and phonons (lattice vibrations) drives the formation of the electron pairs responsible for conventional superconductivity 1 . The lack of direct evidence for electron-phonon coupling in the electron dynamics of the high transition temperature superconductors has driven an intensive search for an alternative mechanism. A coupling of an electron with a phonon would result in an abrupt change of its velocity and scattering rate near the phonon energy. Here we use angle resolved photoemission spectroscopy to probe electron dynamicsvelocity and scattering rate-for three different families of copper oxide superconductors. We see in all of these materials an abrupt change of electron velocity at 50-80meV, which we cannot explain by any known process other than to invoke coupling with the phonons associated with the movement of the oxygen atoms. This suggests that electron-phonon coupling strongly influences the electron dynamics in the high-temperature superconductors, and must therefore be included in any microscopic theory of superconductivity. We investigated the electronic quasiparticle dispersions in three different families of hole-doped cuprates, Bi 2 Sr 2 CaCu 2 O 8 (Bi2212) and Pb doped Pb-Bi2212, Pb-doped Bi 2 Sr 2 CuO 6 (Pb-Bi2201) and La 2-x Sr x CuO 4 (LSCO). Except for the Bi2201 (overdoped, T c =7K) data and that in Fig. 3b, recorded at the beam-line 5.4 of the Stanford Synchrotron Radiation Laboratory (SSRL), all the data were recorded at the Advanced Light Source (ALS), as detailed elsewhere 2 . The top panels of figure 1 report the momentum distribution curve (MDC) derived dispersions along the (0, 0)-(π, π) direction for LSCO (panel a) and Bi2212 (panel b) superconducting state and for Pb-Bi2201 normal state (panel c) vs the rescaled momentum, k ' , defined by normalizing to one the momentum k relative to the Fermi momentum k F , (k-k F ), at the binding energy E=170meV. A "kink" in the dispersion around 50-80meV, highlighted by thick arrows in the figure, is the many-body effect of
Quasiparticle dispersion in Bi2Sr2CaCu2O8 is investigated with improved angular resolution as a function of temperature and doping. Unlike the linear dispersion predicted by the band calculation, the data show a sharp break in dispersion at 50+/-15 meV binding energy where the velocity changes by a factor of 2 or more. This change provides an energy scale in the quasiparticle self-energy. This break in dispersion is evident at and away from the d-wave node line, but the magnitude of the dispersion change decreases with temperature and with increasing doping.
Angle-resolved photoemission spectroscopy was carried out on (La(1.28)Nd(0.6) Sr(0.12))CuO(4), a model system of the charge- and spin-ordered state, or stripe phase. The electronic structure contains characteristic features consistent with other cuprates, such as the flat band at low energy near the Brillouin zone face. However, the low-energy excitation near the expected d-wave node region is strongly suppressed. The frequency-integrated spectral weight is confined inside one-dimensional segments in the momentum space (defined by horizontal momenta &cjs3539;k(x)&cjs3539; = pi/4 and vertical momenta &cjs3539;k(y)&cjs3539; = pi/4), deviating strongly from the more rounded Fermi surface expected from band calculations. This departure from the two-dimensional Fermi surface persists to a very high energy scale. These results provide important information for establishing a theory to understand the charge and spin ordering in cuprates and their relation with high-temperature superconductivity.
High resolution angle-resolved photoemission measurements have been carried out on (La(1.4--x)-Nd(0.6)Sr(x))CuO(4), a model system with static one-dimensional (1D) charge ordering (stripe), and (La(1.85)-Sr(0.15))CuO(4), a high temperature superconductor (T(c) = 40 K) with possible dynamic stripes. In addition to the straight segments near ( pi,0) and ( 0,pi) antinodal regions, we have identified the existence of spectral weight along the [1,1] nodal direction in the electronic structure of both systems. This observation of nodal state, together with the straight segments near antinodal regions, reveals the dual nature of the electronic structure of stripes due to the competition of order and disorder.
C60 fullerides are challenging systems because both the electron-phonon and electron-electron interactions are large on the energy scale of the expected narrow band width. We report angle-resolved photoemission data on the band dispersion for an alkali-doped C60 monolayer and a detailed comparison with theory. Compared to the maximum bare theoretical band width of 170 meV, the observed 100-meV dispersion is within the range of renormalization by electron-phonon coupling. This dispersion is only a fraction of the integrated peak width, revealing the importance of many-body effects. Additionally, measurements on the Fermi surface indicate the robustness of the Luttinger theorem even for materials with strong interactions.
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