The diode effect is fundamental to electronic devices and is widely used in rectifiers and AC-DC converters. At low temperatures, however, conventional semiconductor diodes possess a high resistivity, which yields energy loss and heating during operation. The superconducting diode effect (SDE) 1-8 , which relies on broken inversion symmetry in a superconductor may mitigate this obstacle: in one direction a zero-resistance supercurrent can flow through the diode, but for the opposite direction of current flow, the device enters the normal state with ohmic resistance. The application of a magnetic field can induce SDE inNb/V/Ta superlattices with a polar structure 1,2 , in superconducting devices with asymmetric patterning of pinning centres 9 , or in superconductor/ferromagnet hybrid devices with induced vortices 10,11 . The need for an external magnetic field limits their practical application. Recently, a field-free SDE was observed in a NbSe2/Nb3Br8/NbSe2 junction, and it originates from asymmetric Josephson tunneling that is induced by the Nb3Br8 barrier and the associated NbSe2/Nb3Br8 interfaces 12 . Here, we present another implementation of zero-field SDE using noncentrosymmetric [Nb/V/Co/V/Ta]20 multilayers. The magnetic layers provide the necessary symmetry breaking and we can tune the SDE by adjusting the structural parameters, such as the constituent elements, film thickness, stacking order, and number of repetitions. We control the polarity of the SDE through the magnetization direction of the ferromagnetic layers. Artificially stacked structures 13-18 , as the one used in this work, are of particular interest as they are compatible with microfabrication techniques and can be integrated with devices such as Josephson junctions 19-22 . Energy-loss-free SDEs as presented in this work may therefore enable novel non-volatile memories and logic circuits with ultralow power consumption.
We report that the superconducting critical magnetic field can be nonreciprocal under a bias of an electric current in a superconducting [Nb/V/Ta] n superlattice without a center of inversion. The critical magnetic field showed a clear difference between positive and negative magnetic fields. Furthermore, the magnitude relation between the positive and negative critical magnetic fields is reversed when the direction of the electric current is reversed. Our findings indicate that the superconducting gap can be anisotropic by the application of an electric current.
Recently, an ultimate diode effect, a superconducting diode where an electric current shows the superconducting state in one direction and the normal state in the other direction, has been discovered in a noncentrosymmetric Nb/V/Ta superlattice. Here, we report that the polarity of the superconducting diode shows a sign reversal as a magnetic field is increased. Such a nonlinear behavior of the diode effect is beyond the phenomenology based on the Ginzburg-Landau theory. Based on a recent microscopic study, we propose the crossover and phase transitions of the finite-momentum pairing states as a possible origin of the sign reversals.
Artificially engineered superlattice offers highly flexible control of the quantized electronic state by manipulating its lattice structure. We fabricated artificially engineered superlattices [Nb/V/Ta] n as a new class of superconducting superlattices and investigated the upper critical field H c2 in terms of the structural difference. It is found that the out-of-plane upper critical field H c 2 ⊥ significantly increases compared with that of a Nb single layer film as the thickness of the constituent Nb, V, and Ta layers becomes thin. In the case of the superlattice [Nb/V/Ta] n , the H c 2 ⊥ is basically governed by the orbital pair-breaking effect rather than Pauli pair-breaking effect and increases only when the crystalline size of the superlattice decreases by the insertion of V layers. Thus, we conclude that the shortening of the coherence length of Cooper pairs due to the crystalline disorder predominantly contributes to the increase of the H c 2 ⊥ in the superlattice [Nb/V/Ta] n .
The superconducting diode effect in which electrical resistance is zero in only one direction has recently been reported in superconductors without inversion symmetry. Previous studies investigated the nonreciprocity of the critical current, but little has been known about the rectification effect when AC currents are applied. Herein, we examined the rectification characteristics of a non-centrosymmetric Nb/V/Ta artificial superlattice under AC currents. The rectification strength can be modulated by an applied magnetic field, and its polarity can be tuned by the magnetic field. Furthermore, we find that the magnetic field dependence of the rectification is different from that of the nonreciprocal critical current.
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