We study heterostructures of singlet superconductors and strongly spin-polarized ferromagnets and show that a relative phase arises between the superconducting proximity amplitudes in the two ferromagnetic spin bands. We find a tunable pure spin supercurrent in a spin-polarized ferromagnet contacted with only one superconductor electrode. We show that Josephson junctions are most effective for a spin polarization P approximately 0.3, and that critical currents for positive and negative bias differ for a high transmission Josephson junction, due to a relative phase between single and double pair transmission.

We investigate the mutual proximity effect in a normal metal contacted to a superconductor through a magnetic interface. Analytical and self-consistent numerical results are presented, and we consider both the diffusive and ballistic regimes. We focus on the density of states in both the normal and superconducting region, and find that the presence of spin-dependent phase-shifts occurring at the interface qualitatively modifies the density of states. In particular, we find that the proximity-induced pairing amplitudes in the normal metal region undergo a conversion at the Fermi level from pure even-frequency to odd-frequency. Above a critical value of the interface spin-polarization (or, equivalently, for fixed interface spin-polarization, above a critical interface resistance), only odd frequency correlations remain. This is accompanied by the replacement of the familiar proximity minigap or pseudogap in the normal layer by an enhancement of the density of states above its normal state value for energies near the chemical potential. The robustness of this effect towards inelastic scattering, impurity scattering, and the depletion of the superconducting order parameter close to the interface is investigated. We also study the inverse proximity effect in the diffusive limit. We find that the above-mentioned conversion persists also for thin superconducting layers comparable in size to the superconducting coherence length ξS, as long as the inverse proximity effect is relatively weak. Concomitantly, we find a shift in the critical interface resistance where the pairing conversion occurs. Our findings suggest a robust and simple method for producing purely odd-frequency superconducting correlations, that can be tested experimentally.

We report an extensive theoretical analysis of point-contact Andreev reflection data available in the literature on ferromagnetic CrO2. We find that the spectra can be well understood within a model of fully spin-polarized bands in CrO2 together with spin-active scattering at the contact. This is in contrast to analysis of the data within extended Blonder-Tinkham-Klapwijk models, which lead to a spin polarization varying between 50% and 100% depending on the transparency of the interface. We propose to utilize both the temperature dependence of the spectra and the excess current at voltages above the gap to resolve the spin polarization in CrO2 in a new generation of experiments.

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We study the impact of spin-active scattering on Andreev spectra of point contacts between superconductors(SCs) and strongly spin-polarized ferromagnets(FMs) using recently derived boundary conditions for the Quasiclassical Theory of Superconductivity. We describe the interface region by a microscopic model for the interface scattering matrix. Our model includes both spin-filtering and spin-mixing and is non-perturbative in both transmission and spin polarization. We emphasize the importance of spin-mixing caused by interface scattering, which has been shown to be crucial for the creation of exotic pairing correlations in such structures. We provide estimates for the possible magnitude of this effect in different scenarios and discuss its dependence on various physical parameters. Our main finding is that the shape of the interface potential has a tremendous impact on the magnitude of the spin-mixing effect. Thus, all previous calculations, being based on delta-function or box-shaped interface potentials, underestimate this effect gravely. As a consequence, we find that with realistic interface potentials the spin-mixing effect can easily be large enough to cause spin-polarized sub-gap Andreev bound states in SC/sFM point contacts. In addition, we show that our theory generalizes earlier models based on the Blonder-Tinkham-Klapwijk approach.