Hybrid organic-inorganic compounds are receiving considerable attention in recent years due to the possibility of combining the different characteristics of the components to get unusual and enormous variety of interesting structural topologies and wide potential applications in the fields of catalysis, non-linear optics, sensors, magnetism and molecular recognition [1] . During our investigation, we synthesized three new hybrid organic-inorganic compounds of dapsone with antibacterial and second-order nonlinear optical properties [2] . The structural study and Hirshfeld surface analysis allowed us to establish the importance of hydrogen bond and intermolecular interaction in the crystal packing.and their role in the NLO properties.
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