Electron gases at the surfaces of (001), (110), and (111) oriented SrTiO 3 (STO) have been created using Ar + -irradiation with fully metallic behavior and low-temperature-mobility as large as 5500 cm 2 V -1 s -1 , 1300 cm 2 V -1 s -1 and 8600 cm 2 V -1 s -1 for (001)-, (110)-, and (111)surfaces, respectively. The in-plane anisotropic magnetoresistance (AMR) have been studied for the samples with the current along different crystal axis directions to subtract the Lorentz Force effect. The AMR shows features which coincide with the fixed orientations to the crystalline axes, with 4-fold, 2-fold and nearly-6-fold symmetries for (001)-, (110) and (111)surfaces, respectively, independent of the current directions. These features are possibly caused by the polarization of spin orbit texture of the 2D Fermi surfaces. In addition, a 6-fold to 2-fold symmetry breaking for (111)-surfaces is observed. Our results demonstrate the effect of symmetry of two-dimensional electronic structure on the transport behaviors for the electron gases at STO surfaces.
We report the epitaxial growth of Bi 2 Se 3 thin films on (0001) Al 2 O 3 substrates by hybrid physicalchemical vapor deposition (HPCVD). The HPCVD technique combines the thermal decomposition of trimethylbismuth with the thermal evaporation of Se and leads to a high Se partial pressure in the growth ambient. The Bi 2 Se 3 films are highly c-axis oriented on sapphire but contain planar defects including stacking faults and twin boundaries. Variable-temperature Hall-effect measurements demonstrate a carrier concentration of 5.8 Â 10 18 cm À3 and a mobility of 900 cm 2 /Vs at 4.2 K. These results demonstrate the potential of HPCVD for producing high quality Bi 2 Se 3 films for topological insulator studies. V C 2012 American Institute of Physics. [http://dx.
Proximity-effect-induced superconductivity was studied in epitaxial topological insulator Bi2Se3 thin films grown on superconducting NbSe2 single crystals. A point contact spectroscopy (PCS) method was used at low temperatures down to 40 mK. An induced superconducting gap in Bi2Se3 was observed in the spectra, which decreased with increasing Bi2Se3 layer thickness, consistent with the proximity effect in the bulk states of Bi2Se3 induced by NbSe2. At very low temperatures, an extra point contact feature which may correspond to a second energy gap appeared in the spectrum. For a 16 quintuple layer Bi2Se3 on NbSe2 sample, the bulk state gap value near the top surface is ~159 μeV, while the second gap value is ~120 μeV at 40 mK. The second gap value decreased with increasing Bi2Se3 layer thickness, but the ratio between the second gap and the bulk state gap remained about the same for different Bi2Se3 thicknesses. It is plausible that this is due to superconductivity in Bi2Se3 topological surface states induced through the bulk states. The two induced gaps in the PCS measurement are consistent with the three-dimensional bulk state and the two-dimensional surface state superconducting gaps observed in the angle-resolved photoemission spectroscopy (ARPES) measurement.
Three dimensional topological insulators are characterized by Dirac-like conducting surface states, the existence of which has been confirmed in relatively clean metallic samples by angle-resolved photoemission spectroscopy, as well as by anomalous Aharonov-Bohm oscillations in the magneto-resistance of nanoribbons. However, a fundamental aspect of these surface states, namely their robustness to time-reversal invariant disorder, has remained relatively untested. In this work, we have synthesized thin nanotubes of Bi 2 Te 3 with extremely insulating bulk at low temperatures due to disorder. Nonetheless, the magneto-resistance exhibits quantum oscillations as a function of the magnetic field along the axis of the nanotubes, with a period determined by the cross-sectional area of the outer surface. Detailed numerical simulations based on a recursive Green function method support that the resistance oscillations are arising from the topological surface states which have substantially longer localization length than that of other non-topological states. This observation demonstrates coherent transport at the surface even for highly disordered samples, thus providing a direct confirmation of the inherently topological character of surface states. The result also demonstrates a viable route for revealing the properties of topological states by suppressing the bulk conduction using disorder.3
We report on the thermal and thermoelectric properties of individual nanocrystalline Bi 2 Te 3 nanotubes synthesized by the solution phase method using 3ω method and a microfabricated testbench. Measurements show that the nanotubes offer improved ZT compared to bulk Bi 2 Te 3 near room temperature due to an enhanced Seebeck coefficient and suppressed thermal conductivity. This improvement in ZT originates from the nanocrystalline nature and low dimensionality of the nanotubes. Domain boundary filtering of low-energy electrons provides an enhanced Seebeck coefficient. The scattering of phonons at the surface of the nanotube leads to suppressed thermal conductivity. These have been theoretically analyzed using the Boltzmann equation based on the relaxation time approximation and Landauer approach. This work clearly demonstrates the possibility of achieving enhancement in thermoelectric efficiency by combining nanocrystalline and low-dimensional systems.
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