Few-photon induced breakup of helium is studied using a newly developed ab initio numerical framework for solving the six-dimensional time-dependent Schrödinger equation. We present details of the method and calculate (generalized) cross sections for the process of two-photon nonsequential (direct) double ionization at photon energies ranging from 39.4 to 54.4 eV, a process that has been very much debated in recent years and is not yet fully understood. In particular, we have studied the convergence property of the total cross section in the vicinity of the upper threshold (∼54.4 eV), versus the pulse duration of the applied laser field. We find that the cross section exhibits an increasing trend near the threshold, as has also been observed by others, and show that this rise cannot solely be attributed to an unintended inclusion of the sequential two-photon double ionization process, caused by the bandwidth of the applied field.
We calculate the first-order energy shifts for the N-dimensional hydrogen atom exposed to a static electric field. The results are compared with numerical diagonalization of the Hamiltonian in a finite basis. Using simple scaling relations, we show how corrections to arbitrarily high order may be obtained from known results for the three-dimensional Coulomb problem.
A spatially explicit coupled hydrodynamic-mass transport model system was used to simulate dispersal of particulate organic matter from Atlantic salmon (Salmo salar) farming in central Norway. Model setups of 32 m horizontal resolution were run for periods of up to 650 days for 3 sites of different oceanographic characteristics: one fjord location, one medium-exposed location influenced by fjord water, and one coastal location. Records on feed used for each cage at each location were converted to feces released based on a published mass balance model. The results from the simulations were compared with scores from corresponding mandatory benthic surveys (MOM-B) of the sediment layer beneath the farms. The correspondence between simulated and measured thickness of the sediment layer was good, and improved with the inclusion of resuspension processes. At all sites the distribution of organic matter in the bottom layer was non-homogeneous, with significant temporal variation and transport and settling of matter up to at least 0.5 km away from one of the farms. Our results indicate that the monitoring practice used in Norway until now, with a few sediment grab samples taken mainly within the fish farm, may not adequately determine the areal impacts of all salmon farming operations. The patchy distribution of organic matter and the correspondence between simulation and survey results is attributed to the use of full 3D current fields of a high spatiotemporal resolution and a good model for resuspension processes that some previous model studies have failed to properly account for.
The dynamics of two electrons in a 2-dimensional quantum dot molecule in the presence of a time-dependent electromagnetic field is calculated from first principles. We show that carefully selected microwave pulses can exclusively populate a single state of the first excitation band and that the transition time can be further decreased by optimal pulse control. Finally we demonstrate that an oscillating charge localized state may be created by multiple transitions using a sequence of pulses.
We simulate oil spills of 1500 and 4500m/day lasting 14, 45, and 90days in the spawning grounds of the commercial fish species, Northeast Arctic cod. Modeling the life history of individual fish eggs and larvae, we predict deviations from the historical pattern of recruitment to the adult population due to toxic oil exposures. Reductions in survival for pelagic stages of cod were 0-10%, up to a maximum of 43%. These reductions resulted in a decrease in adult cod biomass of <3% for most scenarios, up to a maximum of 12%. In all simulations, the adult population remained at full reproductive potential with a sufficient number of juveniles surviving to replenish the population. The diverse age distribution helps protect the adult cod population from reductions in a single year's recruitment after a major oil spill. These results provide insights to assist in managing oil spill impacts on fisheries.
We investigate the impact of electron-electron correlation on the ionization dynamics of helium in intense, high-frequency laser fields by solving the time-dependent Schrödinger equation from first principles. Although we observe a decrease in the total ionization yield at high field strengths, the hallmark of atomic stabilization, the repulsion between the electrons has a detrimental effect on the degree of stabilization, in particular for short pulses. Investigation of the ion channel yields reveals that the double ionization process is less prone to two-electron effects, and consequently exhibits the most distinct signature of stabilization. We also find that commonly used one-dimensional models tend to overestimate the effect of correlation.
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