We study the impact of the wetting properties on the immiscible displacement of a viscous fluid in disordered porous media. We present a novel pore-scale model that captures wettability and dynamic effects, including the spatiotemporal nonlocality associated with interface readjustments. Our simulations show that increasing the wettability of the invading fluid (the contact angle) promotes cooperative pore filling that stabilizes the invasion, and that this effect is suppressed as the flow rate increases, due to viscous instabilities. We use scaling analysis to derive two dimensionless numbers that predict the mode of displacement. By elucidating the underlying mechanisms, we explain classical yet intriguing experimental observations. These insights could be used to improve technologies such as hydraulic fracturing, CO2 geo-sequestration, and microfluidics. 47.56.+r, Fluid-fluid displacement in porous media is important in natural and industrial processes at various scales, from enhanced energy recovery, CO 2 geo-sequestration, groundwater contamination and soil wetting and drying, to dyeing of paper or textiles and microfluidics. Fluid displacement is governed by the interplay between quenched disorder, short-range cooperative effects and long-range pressure screening, which depends on a large number of parameters, including the wettability-the relative affinity of the fluids to the solid. Consequently, the displacement patterns can range from a stable, compact front to highly ramified with preferential flow paths (fingers) [1]. Fluid invasion is a member of a broad class of problems characterized by competitive domain growth and nonlinear interface dynamics, including magnetic domains, biological films and flame front propagation [2]. The interface evolution in these systems is often modeled as a competition between the energy associated with the interaction between phases and constraints arising from disorder; the relative importance of the two can be tuned by properties such as wettability in fluid displacement or local random interaction fields in magnetic domains [3]. Understanding the impact of wettability on fluid invasion-the topic of this Letter-is therefore relevant to a wide range of phenomena of scientific and technological importance.Immiscible displacement can be classified according to the wettability into drainage or nonwetting invasion, where the displaced fluid preferentially wets the solid (contact angle θ < 90 • , measured through the defending fluid), or imbibition of a wetting fluid (θ > 90 • ). Intensive research has provided basic understanding of drainage, identifying different invasion behaviors and explaining their dependence on the flow velocity, fluid viscosities, interfacial tension, and the degree of porescale disorder ([4-7] and the references therein). Increasing θ was found to stabilize the displacement and reduce trapping in forced and gravity-driven drainage experiments [8,9].In contrast, relatively few works have studied imbibition, mostly for the stable case of a more vis...
Multiphase flows in porous media are important in many natural and industrial processes. Pore-scale models for multiphase flows have seen rapid development in recent years and are becoming increasingly useful as predictive tools in both academic and industrial applications. However, quantitative comparisons between different pore-scale models, and between these models and experimental data, are lacking. Here, we perform an objective comparison of a variety of state-of-the-art pore-scale models, including lattice Boltzmann, stochastic rotation dynamics, volume-of-fluid, level-set, phase-field, and pore-network models. As the basis for this comparison, we use a dataset from recent microfluidic experiments with precisely controlled pore geometry and wettability conditions, which offers an unprecedented benchmarking opportunity. We compare the results of the 14 participating teams both qualitatively and quantitatively using several standard metrics, such as fractal dimension, finger width, and displacement efficiency. We find that no single method excels across all conditions and that thin films and corner flow present substantial modeling and computational challenges.
We study the displacement of immiscible fluids in deformable, noncohesive granular media. Experimentally, we inject air into a thin bed of water-saturated glass beads and observe the invasion morphology. The control parameters are the injection rate, the bead size, and the confining stress. We identify three invasion regimes: capillary fingering, viscous fingering, and "capillary fracturing," where capillary forces overcome frictional resistance and induce the opening of conduits. We derive two dimensionless numbers that govern the transition among the different regimes: a modified capillary number and a fracturing number. The experiments and analysis predict the emergence of fracturing in fine-grained media under low confining stress, a phenomenon that likely plays a fundamental role in many natural processes such as primary oil migration, methane venting from lake sediments, and the formation of desiccation cracks.
We present a systematic, quantitative assessment of the impact of pore size disorder and its interplay with flow rates and wettability on immiscible displacement of a viscous fluid. Pore-scale simulations and micromodel experiments show that reducing disorder increases the displacement efficiency and compactness, minimizing the fluid-fluid interfacial area, through (i) trapping at low rates and (ii) viscous fingering at high rates. Increasing the wetting angle suppresses both trapping and fingering, hence reducing the sensitivity of the displacement to the underlying disorder. A modified capillary number Ca* that includes the impact of disorder λ on viscous forces (through pore connectivity) is direct related to λ, in par with previous works. Our findings bear important consequences on sweep efficiency and fluid mixing and reactions, which are key in applications such as microfluidics to carbon geosequestration, energy recovery, and soil aeration and remediation.
We investigate the displacement of one fluid by another in a deformable medium with pore-scale disorder. We develop a model that captures the dynamic pressure redistribution at the invasion front and the feedback between fluid invasion and microstructure rearrangement. Our results suggest how to collapse the transition between invasion percolation and viscous fingering in the presence of quenched disorder. We predict the emergence of a fracturing pattern for sufficiently deformable media, in agreement with observations of drainage in granular material. We identify a dimensionless number that appears to govern the crossover from fingering to fracturing.
Abstract. We study the relation between surface infiltration and groundwater recharge during managed aquifer recharge (MAR) with desalinated seawater in an infiltration pond, at the Menashe site that overlies the northern part of the Israeli Coastal Aquifer. We monitor infiltration dynamics at multiple scales (up to the scale of the entire pond) by measuring the ponding depth, sediment water content and groundwater levels, using pressure sensors, single-ring infiltrometers, soil sensors, and observation wells. During a month (January 2015) of continuous intensive MAR (2.45 × 10 6 m 3 discharged to a 10.7 ha area), groundwater level has risen by 17 m attaining full connection with the pond, while average infiltration rates declined by almost 2 orders of magnitude (from ∼ 11 to ∼ 0.4 m d −1 ). This reduction can be explained solely by the lithology of the unsaturated zone that includes relatively low-permeability sediments. Clogging processes at the pond-surface -abundant in many MAR operations -are negated by the high-quality desalinated seawater (turbidity ∼ 0.2 NTU, total dissolved solids ∼ 120 mg L −1 ) or negligible compared to the low-permeability layers. Recharge during infiltration was estimated reasonably well by simple analytical models, whereas a numerical model was used for estimating groundwater recharge after the end of infiltration. It was found that a calibrated numerical model with a onedimensional representative sediment profile is able to capture MAR dynamics, including temporal reduction of infiltration rates, drainage and groundwater recharge. Measured infiltration rates of an independent MAR event (January 2016) fitted well to those calculated by the calibrated numerical model, showing the model validity. The successful quantification methodologies of the temporal groundwater recharge are useful for MAR practitioners and can serve as an input for groundwater flow models.
SUMMARYThe mechanical properties of cohesionless granular materials are evaluated from grain-scale simulations. A three-dimensional pack of spherical grains is loaded by incremental displacements of its boundaries. The deformation is described as a sequence of equilibrium configurations. Each configuration is characterized by a minimum of the total potential energy. This minimum is computed using a modification of the conjugate gradient algorithm.Our simulations capture the nonlinear, path-dependent behavior of granular materials observed in experiments. Micromechanical analysis provides valuable insight into phenomena such as hysteresis, strain hardening and stress-induced anisotropy. Estimates of the effective bulk modulus, obtained with no adjustment of material parameters, are in agreement with published experimental data. The model is applied to evaluate the effects of hydrate dissociation in marine sediments. Weakening of the sediment is quantified as a reduction in the effective elastic moduli.
We study the effect of spatially‐correlated heterogeneity on isothermal drying of porous media. We combine a minimal pore‐scale model with microfluidic experiments with the same pore geometry. Our simulated drying behavior compares favorably with experiments, considering the large sensitivity of the emergent behavior to the uncertainty associated with even small manufacturing errors. We show that increasing the correlation length in particle sizes promotes preferential drying of clusters of large pores, prolonging liquid connectivity and surface wetness and thus higher drying rates for longer periods. Our findings improve our quantitative understanding of how pore‐scale heterogeneity impacts drying, which plays a role in a wide range of processes ranging from fuel cells to curing of paints and cements to global budgets of energy, water and solutes in soils.
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