A simple experiment is descried here that has become extremely popular in chemical research because it can provide useful information about redox reactions in a form that is easily obtained and interpreted. In this paper the authors present the principles of the method and illustrate its use in the study of four electrode reactions. From State-of-the-Art Symposium: Electrochemistry, ACS meeting, Kansas City, 1982.
This paper reviews the impact of World Meteorological Organization (WMO) Aircraft Meteorological Data Relay (AMDAR) observations on operational numerical weather prediction (NWP) forecasts at both regional and global scales that support national and local weather forecast offices across the globe. Over the past three decades, data collected from commercial aircraft have helped reduce flight-level wind and temperature forecast errors by nearly 50%. Improvements are largest in 3–48-h forecasts and in regions where the automated reports 1) are most numerous, 2) cover a broad area, and 3) are available at multiple levels (e.g., made during aircraft ascent and descent). Improvements in weather forecasts due to these data have already had major impacts on a variety of aspects of airline operations, ranging from fuel savings from improved wind and temperature forecasts used in flight planning to passenger comfort and safety due to better awareness of en route and near-terminal weather hazards. Aircraft wind and temperature observations now constitute the third most important dataset for global NWP and, in areas of ample reports, have become the single most important dataset for use in shorter-term, regional NWP applications. Automated aircraft reports provide the most cost-effective data source for improving NWP, being more than 5 times more cost effective than any other major-impact observing system. They also present an economical alternative for obtaining tropospheric profiles both in areas of diminishing conventional observation and as a supplement to existing datasets, both in time and space. An evaluation of moisture observations becoming available from an increasing number of AMDAR-equipped aircraft will be presented in Part II of this paper, including examples of the use of the full array of AMDAR observations in a variety of forecasting situations.
Geostationary satellite-derived atmospheric motion vectors (AMVs) have been used over several decades in a wide variety of meteorological applications. The ever-increasing horizontal and vertical resolution of numerical weather prediction models puts a greater demand on satellite-derived wind products to monitor flow accurately at smaller scales and higher temporal resolution. The focus of this paper is to evaluate the accuracy and potential applications of a newly developed experimental mesoscale AMV product derived from Geostationary Operational Environmental Satellite (GOES) imagery. The mesoscale AMV product is derived through a variant on processing methods used within the University of Wisconsin-Madison Cooperative Institute for Meteorological Satellite Studies (UW-CIMSS) AMV algorithm and features a significant increase in vector density throughout the troposphere and lower stratosphere over current NOAA/ National Environmental Satellite, Data, and Information Service (NESDIS) processing methods for GOES-12 Imager data. The primary objectives of this paper are to 1) highlight applications of experimental GOES mesoscale AMVs toward weather diagnosis and forecasting, 2) compare the coverage and accuracy of mesoscale AMVs with the NOAA/NESDIS operational AMV product, and 3) demonstrate the utility of 6-min NOAA Wind Profiler Network observations for satellite-derived AMV validation. Although the more conservative NOAA/NESDIS AMV product exhibits closer statistical agreement to rawinsonde and wind profiler observations than do the experimental mesoscale AMVs, a comparison of these two products for selected events shows that the mesoscale product better depicts the circulation center of a midlatitude cyclone, boundary layer confluence patterns, and a narrow low-level jet that is well correlated with subsequent severe thunderstorm development. Thus, while the individual experimental mesoscale AMVs may sacrifice some absolute accuracy, they show promise in providing greater temporal and spatial flow detail that can benefit diagnosis of upper-air flow patterns in near-real time. The results also show good agreement between 6-min wind profiler and rawinsonde observations within the 700-200-hPa layer, with larger differences in the stratosphere, near the mean top of the planetary boundary layer, and just above the earth's surface. Despite these larger differences within select layers, the stability of the difference profile with height builds confidence in the use of 6-min, ;404-MHz NOAA Wind Profiler Network observations to evaluate and better understand satellite AMV error characteristics.
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