Thin films of ferromagnetic (Fe70Ni30)96Mo4 were grown via molecular beam epitaxy. Their magnetic properties and magnetocaloric effects were investigated. X-ray diffraction and vibrating sample magnetometry measurements confirmed the crystalline ferromagnetic (Fe70Ni30)96Mo4 phase, with a Curie point near room temperature. To determine the suitability of this material for magnetocaloric applications, we observed a large magnetic entropy change with a large temperature span as well as high relative cooling power near Curie temperature comparable to rare-earth-based materials operating near room temperature.

Thin films of ferromagnet Fe2Ge were grown via molecular beam epitaxy, and their electrical and magneto-transport properties were measured for the first time. X-ray diffraction and vibrating sample magnetometry measurements confirmed the crystalline ferromagnetic Fe2Ge phase. The observed high-temperature maximum in the longitudinal resistivity, as well as the observed suppression of electron–magnon scattering at low temperatures, points to the presence of strong spin polarization in this material. Measurements of the Hall resistivity, ρxy, show contributions from both the ordinary Hall effect and the anomalous Hall effect, ρxyAH, from which we determined the charge carrier concentration and mobility. Measurements also show a small negative magnetoresistance in both the longitudinal and transverse geometries. Fe2Ge holds promise as a useful spintronic material, especially for its semiconductor compatibility.

Thin films of iron–tin alloy FeSn are grown on silicon substrates and their structural and transport properties are investigated for the first time. Herein, the molecular beam epitaxy method is used to grow 50 and 30 nm thick FeSn films on silicon substrates containing 10 nm of MgO as a buffer layer. The films are characterized structurally using an X‐ray diffractometer, showing a hexagonal crystal structure with the space group P6/mmm (191). The results from electrical and magnetotransport measurements show these films exhibit characteristics close to metals. Herein, the magnetotransport properties of the thin films which show positive magnetoresistance and sample‐dependent Hall effect with possible multiband transport are further measured.