Methane (CH4) emissions from natural gas production are not well quantified and have the potential to offset the climate benefits of natural gas over other fossil fuels. We use atmospheric measurements in a mass balance approach to estimate CH4 emissions of 55 ± 15 × 103 kg h−1 from a natural gas and oil production field in Uintah County, Utah, on 1 day: 3 February 2012. This emission rate corresponds to 6.2%–11.7% (1σ) of average hourly natural gas production in Uintah County in the month of February. This study demonstrates the mass balance technique as a valuable tool for estimating emissions from oil and gas production regions and illustrates the need for further atmospheric measurements to determine the representativeness of our single‐day estimate and to better assess inventories of CH4 emissions.

The California Research at the Nexus of Air Quality and Climate Change (CalNex) field study was conducted throughout California in May, June, and July of 2010. The study was organized to address issues simultaneously relevant to atmospheric pollution and climate change, including (1) emission inventory assessment, (2) atmospheric transport and dispersion, (3) atmospheric chemical processing, and (4) cloud‐aerosol interactions and aerosol radiative effects. Measurements from networks of ground sites, a research ship, tall towers, balloon‐borne ozonesondes, multiple aircraft, and satellites provided in situ and remotely sensed data on trace pollutant and greenhouse gas concentrations, aerosol chemical composition and microphysical properties, cloud microphysics, and meteorological parameters. This overview report provides operational information for the variety of sites, platforms, and measurements, their joint deployment strategy, and summarizes findings that have resulted from the collaborative analyses of the CalNex field study. Climate‐relevant findings from CalNex include that leakage from natural gas infrastructure may account for the excess of observed methane over emission estimates in Los Angeles. Air‐quality relevant findings include the following: mobile fleet VOC significantly declines, and NOx emissions continue to have an impact on ozone in the Los Angeles basin; the relative contributions of diesel and gasoline emission to secondary organic aerosol are not fully understood; and nighttime NO3 chemistry contributes significantly to secondary organic aerosol mass in the San Joaquin Valley. Findings simultaneously relevant to climate and air quality include the following: marine vessel emissions changes due to fuel sulfur and speed controls result in a net warming effect but have substantial positive impacts on local air quality.

[1] In the summer of 2004 several separate field programs intensively studied the photochemical, heterogeneous chemical and radiative environment of the troposphere over North America, the North Atlantic Ocean, and western Europe. Previous studies have indicated that the transport of continental emissions, particularly from North America, influences the concentrations of trace species in the troposphere over the North Atlantic and Europe. An international team of scientists, representing over 100 laboratories, collaborated under the International Consortium for Atmospheric Research on Transport and Transformation (ICARTT) umbrella to coordinate the separate field programs in order to maximize the resulting advances in our understanding of regional air quality, the transport, chemical transformation and removal of aerosols, ozone, and their precursors during intercontinental transport, and the radiation balance of the troposphere. Participants utilized nine aircraft, one research vessel, several ground-based sites in North America and the Azores, a network of aerosol-ozone lidars in Europe, satellites, balloon borne sondes, and routine commercial aircraft measurements. In this special section, the results from a major fraction of those platforms are presented. This overview is aimed at providing operational and logistical information for those platforms, summarizing the principal findings and conclusions that have been drawn from the results, and directing readers to specific papers for further details.

The concept of boundary layer mixing height for meteorology and air quality applications using lidar data is reviewed, and new algorithms for estimation of mixing heights from various types of lower-tropospheric coherent Doppler lidar measurements are presented. Velocity variance profiles derived from Doppler lidar data demonstrate direct application to mixing height estimation, while other types of lidar profiles demonstrate relationships to the variance profiles and thus may also be used in the mixing height estimate. The algorithms are applied to ship-based, high-resolution Doppler lidar (HRDL) velocity and backscattered-signal measurements acquired on the R/V Ronald H. Brown during Texas Air Quality Study (TexAQS) 2006 to demonstrate the method and to produce mixing height estimates for that experiment. These combinations of Doppler lidar–derived velocity measurements have not previously been applied to analysis of boundary layer mixing height—over the water or elsewhere. A comparison of the results to those derived from ship-launched, balloon-radiosonde potential temperature and relative humidity profiles is presented.

The Second Texas Air Quality Study (TexAQS II) was conducted in eastern Texas during 2005 and 2006. This 2‐year study included an intensive field campaign, TexAQS 2006/Gulf of Mexico Atmospheric Composition and Climate Study (GoMACCS), conducted in August–October 2006. The results reported in this special journal section are based on observations collected on four aircraft, one research vessel, networks of ground‐based air quality and meteorological (surface and radar wind profiler) sites in eastern Texas, a balloon‐borne ozonesonde‐radiosonde network (part of Intercontinental Transport Experiment Ozonesonde Network Study (IONS‐06)), and satellites. This overview paper provides operational and logistical information for those platforms and sites, summarizes the principal findings and conclusions that have thus far been drawn from the results, and directs readers to appropriate papers for the full analysis. Two of these findings deserve particular emphasis. First, despite decreases in actual emissions of highly reactive volatile organic compounds (HRVOC) and some improvements in inventory estimates since the TexAQS 2000 study, the current Houston area emission inventories still underestimate HRVOC emissions by approximately 1 order of magnitude. Second, the background ozone in eastern Texas, which represents the minimum ozone concentration that is likely achievable through only local controls, can approach or exceed the current National Ambient Air Quality Standard of 75 ppbv for an 8‐h average. These findings have broad implications for air quality control strategies in eastern Texas.

A review of remote sensing technology for lower tropospheric thermodynamic (TD) profiling is presented with focus on high accuracy and high temporal-vertical resolution. The contributions of these instruments to the understanding of the Earth system are assessed with respect to radiative transfer, land surface-atmosphere feedback, convection initiation, and data assimilation. We demonstrate that for progress in weather and climate research, TD profilers are essential. These observational systems must resolve gradients of humidity and temperature in the stable or unstable atmospheric surface layer close to the ground, in the mixed layer, in the interfacial layer-usually characterized by an inversion-and the lower troposphere. A thorough analysis of the current observing systems is performed revealing significant gaps that must be addressed to fulfill existing needs. We analyze whether current and future passive and active remote sensing systems can close these gaps. A methodological analysis and demonstration of measurement capabilities with respect to bias and precision is executed both for passive and active remote sensing including passive infrared and microwave spectroscopy, the global navigation satellite system, as well as water vapor and temperature Raman lidar and water vapor differential absorption lidar. Whereas passive remote sensing systems are already mature with respect to operational applications, active remote sensing systems require further engineering to become operational in networks. However, active remote sensing systems provide a smaller bias as well as higher temporal and vertical resolutions. For a suitable mesoscale network design, TD profiler system developments should be intensified and dedicated observing system simulation experiments should be performed.

The influence of stratosphere‐to‐troposphere transport (STT) on surface ozone (O3) concentrations in the greater Los Angeles area during the CalNex and IONS‐2010 measurement campaigns has been investigated. Principal component analysis (PCA) of surface O3measurements from 41 sampling stations indicates that ∼13% of the variance in the maximum daily 8‐h average (MDA8) O3between May 10 and June 19, 2010 was associated with changes of 2–3 day duration linked to the passage of upper‐level troughs. Ozonesondes launched from Joshua Tree National Park and airborne lidar measurements show that these changes coincided with the appearance of stratospheric intrusions in the lower troposphere above southern California. The Lagrangian particle dispersion model FLEXPART reproduces most of these intrusions, and supports the conclusion from the PCA that significant transport of stratospheric air to the surface occurred on May 28–30. This intrusion led to a peak 1‐h O3 concentration of 88 ppbv at Joshua Tree National Monument near the ozonesonde launch site on May 28, and widespread entrainment of stratospheric air into the boundary layer increased the local background O3 over the entire area to ∼55 ppbv on May 29–30. This background was 10–15 ppbv higher than the baseline O3 in air transported ashore from the Pacific Ocean, and when combined with locally produced O3 led to several exceedances of the current National Ambient Air Quality Standard (NAAQS) on the following day.

Atmospheric variables in the convective boundary layer (CBL), which are critical for turbulence parameterizations in weather and climate models, are assessed. These include entrainment fluxes, higher-order moments of humidity, potential temperature, and vertical wind, as well as dissipation rates. Theoretical relationships between the integral scales, gradients, and higher-order moments of atmospheric variables, fluxes, and dissipation rates are developed mainly focusing on the entrainment layer (EL) at the top of the CBL. These equations form the starting point for tests of and new approaches in CBL turbulence parameterizations. For the investigation of these relationships, an observational approach using a synergy of ground-based water vapor, temperature, and wind lidar systems is proposed. These systems measure instantaneous vertical profiles with high temporal and spatial resolution throughout the CBL including the EL. The resolution of these systems permits the simultaneous measurement of gradients and fluctuations of these atmospheric variables. For accurate analyses of the gradients and the shapes of turbulence profiles, the lidar system performances are very important. It is shown that each lidar profile can be characterized very well with respect to bias and system noise and that the constant bias has negligible effect on the measurement of turbulent fluctuations. It is demonstrated how different gradient relationships can be measured and tested with the proposed lidar synergy within operational measurements or new field campaigns. Particularly, a novel approach is introduced for measuring the rate of destruction of humidity and temperature variances, which is an important component of the variance budget equations.