Black phosphorus (BP), an emerging 2D material semiconductor material, exhibits unique properties and promising application prospects for photo/ electrocatalysis. However, the applications of BP in photo/electrocatalysis are hampered by the instability as well as low catalysis efficiency. Recently, tremendous efforts have been dedicated toward modulating its intrinsic structure, electronic property, and charge separation for enhanced photo/ electrocatalytic performance through structure engineering. Simultaneously, the search for new substitute materials that are BP-analogous is ongoing. Herein, the latest theoretical and experimental progress made in the structural/surface engineering strategies and advanced applications of BP and BP-analog materials in relation to photo/electrocatalysis are extensively explored, and a presentation of the future opportunities and challenges of the materials is included at the end.
Pioneered by Google's Pregel, many distributed systems have been developed for large-scale graph analytics. These systems expose the user-friendly "think like a vertex" programming interface to users, and exhibit good horizontal scalability. However, these systems are designed for tasks where the majority of graph vertices participate in computation, but are not suitable for processing lightworkload graph queries where only a small fraction of vertices need to be accessed. The programming paradigm adopted by these systems can seriously under-utilize the resources in a cluster for graph query processing. In this work, we develop a new open-source system, called Quegel, for querying big graphs, which treats queries as first-class citizens in the design of its computing model. Users only need to specify the Pregel-like algorithm for a generic query, and Quegel processes light-workload graph queries on demand using a novel superstep-sharing execution model to effectively utilize the cluster resources. Quegel further provides a convenient interface for constructing graph indexes, which significantly improve query performance but are not supported by existing graph-parallel systems. Our experiments verified that Quegel is highly efficient in answering various types of graph queries and is up to orders of magnitude faster than existing systems.
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