Torque can be provided to magnetization in nanomagnets directly by electric current and/or voltage. This technique enables electric current (voltage)-to-spin conversion without electromagnetic induction, and has been intensively studied for memory device applications. Among the various kinds of torque, torque induced by spin-orbit splitting has recently been found. However, quantitative understanding of bulkrelated torque and interface-related torque is still lacking because of their identical symmetry for currentin-plane devices. In this paper, we propose that a pure interface-related torque can be characterized by spintorque ferromagnetic resonance with a current-perpendicular-to-plane tunnel junction. Epitaxial Fe-MgO-V tunnel junctions are prepared to characterize the interface-related torque at Fe-MgO. We find that the current-driven torque is negligible, and a significant enhancement of the voltage-driven torque is observed when the MgO barrier thickness decreases. The maximum torque obtained is as large as 2.8 × 10 −5 J=ðVm 2 Þ, which is comparable to the voltage-controlled magnetic anisotropy of 180 fJ=Vm. The voltage-driven torque shows strong dc-bias-voltage dependence that cannot be explained by conventional voltage-controlled magnetic anisotropy. Tunnel anisotropic magnetoresistance spectroscopy suggests that the torque is correlated to an interface state at the Fe-MgO. This surface-state-sensitive electric modulation of magnetic properties provides new insight into the field of interface magnetism.

In our proof-of-principle study we examine the influence of skyrmions on magnetoresistive transport. In particular, we show that magnetic tunnel junctions are a technologically appealing and promising way for electrical detection of non-collinear magnetic structures. The calculated effect is shown to originate from scattering between different k-states and cannot be identified through densities of states alone. Our results suggest that the detection efficiency strongly depends on the utilized materials.

Electric control of magnetism has been a topic of interest for various spintronic applications. It is known that monoatomic Pt layer insertion at the Fe/MgO interface increases voltage-controlled magnetic anisotropy (VCMA). However, the reason for the optimality of this thickness has not been explained thus far. In this study, we observed the changes in the electronic states at the Fe/MgO interface using tunneling spectroscopy on an epitaxial Fe(001)/Pt/MgO(001) structure to characterize the density of states around the Fermi level. We found that a surface resonant state is formed at the Fermi level by the insertion of a monoatomic Pt layer, which is consistent with our first principles study. In addition, the VCMA enhancement owing to the formation of this surface resonance state agrees with the recently proposed microscopic theory.

Disorder effects in alloys are usually modeled by averaging various supercell calculations considering different positions of the alloy atoms. This approach, however, is only possible as long as the portion of the individual components of the alloy are sufficiently large. Herein we present an ab initio study considering the lithium insertion material Li1−x[Ni0.33Co0.33Mn0.33]O2 as model system to demonstrate the power of the coherent potential approximation within the Korringa-Kohn-Rostoker Green's function method. This approach enables the description of disorder effects within alloy systems of any composition. It is applied in this study to describe the (de-)intercalation of arbitrary amounts of lithium from the cathode active material. Moreover, we highlight that using either fully optimized structures or experimental lattice parameters and atomic positions both lead to comparable results. Our findings suggest that this approach is also suitable for modeling the electronic structure of state-of-the-art materials such as high-nickel alloys.