Realizing Majorana bound states in chains of magnetic impurities on s-wave superconducting substrates relies on a fine tuning of the energy and hybridization of the single magnetic impurity bound states and of the spin-orbit coupling (SOC). While recent experiments investigate the influence of the former two parameters, the effect of SOC remained experimentally largely unexplored.Here, we present a scanning tunneling spectroscopy study of close-packed Mn chains along the [001]direction on Ta(110) which has almost identical atomic and surface electronic structure compared to the previously studied Nb(110) system, but a three times larger SOC. The dominant Shiba band has a very similar dispersion, but its minigap, taken relative to ∆, is increased by a factor of 1.9 with respect to the Nb case, which can be ascribed to the stronger SOC.
Magnetic adatoms coupled to an s-wave superconductor give rise to local bound states, so-called Yu-Shiba-Rusinov states. Focusing on the ultimate goal of tailoring chains of such adatoms into a topologically superconducting phase, we investigate basic building blocks -single Fe and Mn adatoms and Mn dimers on clean superconducting Ta(110) -using scanning tunneling microscopy and spectroscopy. We perform a systematic study of the hybridizations and splittings in dimers, and their dependence on the crystallographic directions and interatomic spacings, in order to identify potentially interesting chain geometries for this novel sample type. Subsequently, we study the spin structure as well as the length dependent Shiba band structure in Mn chains of those geometries using spin-resolved scanning tunneling spectroscopy. All results are compared to the according properties of structurally identical dimers and chains on the previously studied Nb(110), which has almost identical surface structure and electronic properties, but an about three times smaller spin-orbit interaction.
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