We successfully fabricated a planar nanocomposite film that uses a composite of silver nanoparticles and titanium dioxide film (Ag-TiO2) for ultraviolet (UV) and blue light detection and application in ozone gas sensor. Ultraviolet-visible spectra revealed that silver nanoparticles have a strong surface plasmon resonance (SPR) effect. A strong redshift of the plasmonic peak when the silver nanoparticles covered the TiO2 thin film was observed. The value of conductivity change for the Ag-TiO2 composite is 4–8 times greater than that of TiO2 film under UV and blue light irradiation. The Ag-TiO2 nanocomposite film successfully sensed 100 ppb ozone. The gas response of the composite film increased by roughly six and four times under UV and blue light irradiation, respectively. We demonstrated that a Ag-TiO2 composite gas sensor can be used with visible light (blue). The planar composite significantly enhances photo catalysis. The composite films have practical application potential for wearable devices.
Transition metal dichalcogenides (TMDs) with only a few atoms thickness provide an excellent solution to scale down current semiconductor devices. Many studies have demonstrated that molybdenum disulfide (MoS2), a member of TMDs, is promising as a channel material to fabricate field-effect transistors (FETs). However, the carrier mobility in MoS2 FET is always far lower than the theoretical prediction. Although this poor performance can be attributed to the defects, it still lacks a quantitative analysis clarifying the correlation between carrier mobility and defect density. In this work, by using scanning tunneling microscopy, we directly counted the defects in MoS2 FETs with different carrier mobility. We found that vacancies and impurities equally contribute to carrier mobility and the total defect density induces a power-law decreasing tendency to the carrier mobility of MoS2 FET. Our current results directly prove that the reduction of point defects can exponentially improve the carrier mobility of FETs made by TMDs.
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